Two-dimensional spectroscopy by spectrally resolved real-time resonant coherent Raman scattering in polydiacetylene

被引:0
作者
Ishii, N [1 ]
Tokunaga, E [1 ]
Adachi, S [1 ]
Kimura, T [1 ]
Matsuda, H [1 ]
Kobayashi, T [1 ]
机构
[1] Univ Tokyo, Grad Sch Sci, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan
来源
ULTRAFAST PHENOMENA XIV | 2005年 / 79卷
关键词
D O I
暂无
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Spectrally resolved real-time coherent resonant Raman scattering was observed by a 4-fs ultrashort pulse with a spectrally resolving multi-channel lock-in amplifier and was identified by a theoretical calculation. An introduced optical frequency-and vibrational time-resolved two-dimensional spectrum reveals the electronic ground-state dynamics below the absorption edge.
引用
收藏
页码:563 / 565
页数:3
相关论文
共 5 条
[1]   Visible pulse compression to 4 fs by optical parametric amplification and programmable dispersion control [J].
Baltuska, A ;
Fuji, T ;
Kobayashi, T .
OPTICS LETTERS, 2002, 27 (05) :306-308
[2]   Investigations of amplitude and phase excitation profiles in femtosecond coherence spectroscopy [J].
Kumar, ATN ;
Rosca, F ;
Widom, A ;
Champion, PM .
JOURNAL OF CHEMICAL PHYSICS, 2001, 114 (02) :701-724
[3]   MODELING VIBRATIONAL MODES IN DIACETYLENE POLYMERS [J].
LEWIS, WF ;
BATCHELDER, DN .
CHEMICAL PHYSICS LETTERS, 1979, 60 (02) :232-237
[4]  
Mukamel S., 1999, PRINCIPLES NONLINEAR
[5]   FEMTOSECOND PUMP-PROBE SPECTROSCOPY OF POLYATOMIC-MOLECULES IN CONDENSED PHASES [J].
YAN, YJ ;
MUKAMEL, S .
PHYSICAL REVIEW A, 1990, 41 (11) :6485-6504