Laboratory-Scale Studies on Humidified O2-Fed High-Ash Coal-Based Underground Coal Gasification

被引:6
|
作者
Kashyap, Swarnotpal [1 ]
Vairakannu, Prabu [1 ]
机构
[1] IIT Guwahati, Dept Chem Engn, Gauhati 781039, Assam, India
关键词
POWER-GENERATION; INDIAN COALS; EX-SITU; LIGNITE; CONTEXT; STEAM; MINE; CO2;
D O I
10.1021/acs.energyfuels.8b01854
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
With the depletion of coal reserves all over the world, efforts are being made worldwide to utilize those deep underground coal seams, which are difficult to mine or are not feasible economically. Underground coal gasification (UCG) is a promising technology to achieve that objective and also to reduce the atmospheric pollution that is casued by surface gasification of the mined coal. Based on the previous research performed in this field, it is a well-known fact that the optimum quantity of water influx into coal seam can increase the hydrogen content of the product gas. In our earlier study, a novel method of utilizing humidified oxygen as the gasification agent was conducted for low ash coal gasification. The experimental results had shown the production of substantial quantity of hydrogen in the product gas. In the present study, the laboratory scale experiments are extended to high-ash Indian coals with increases in the absolute humidity of the feed oxygen by preheating the water (humidifying medium) at different temperatures in the range of 30-65 degrees C, with an interval of 5 degrees C. The composition of the product gas composition is estimated for the borehole gasification of high ash and low ash Indian coals with warm humidified oxygen as the feed stream. The optimum preheating temperature for the gasification of low ash and high ash coals is estimated as 45 and 30 degrees C, respectively. The average calorific value of the product gas is found as 239.8 kJ/mol for low-ash coals and 171.2 kJ/mol for high-ash coals. The average hydrogen content in the syngas during low-ash coal gasification is 26.9%, whereas, during high-ash coal gasification, it is 18.1%. The hydrogen gas is obtained as high as 33% for low-ash coals and 28% for high-ash coals.
引用
收藏
页码:9132 / 9141
页数:10
相关论文
共 33 条
  • [21] Studies on NOx formation and reduction characteristics in high-ash, low-volatile coal combustion by mechanism experiments and industrial-scale trials
    Li, Xiaoguang
    Li, Shiyuan
    Li, Zhengqi
    Chen, Zhichao
    Qin, Yukun
    APPLIED THERMAL ENGINEERING, 2024, 256
  • [22] Gasification of Inferior Coal with High Ash Content under CO2 and O2/H2O Atmospheres
    Yang, Zhongqing
    Zhang, Li
    Peng, Jin
    Guo, Mingnv
    INTERNATIONAL JOURNAL OF GREEN ENERGY, 2015, 12 (10) : 1046 - 1053
  • [23] CO2 pyrolysis and gasification of COVID-19 based wastes (overall gown) with Indian high ash coal
    Sahu, Pradeep
    Vairakannu, Prabu
    ASIA-PACIFIC JOURNAL OF CHEMICAL ENGINEERING, 2023, 18 (04)
  • [24] Effect of Injection Flow Rate on Product Gas Quality in Underground Coal Gasification (UCG) Based on Laboratory Scale Experiment: Development of Co-Axial UCG System
    Hamanaka, Akihiro
    Su, Fa-qiang
    Itakura, Ken-ichi
    Takahashi, Kazuhiro
    Kodama, Jun-ichi
    Deguchi, Gota
    ENERGIES, 2017, 10 (02):
  • [25] Experimental and kinetic studies on in-situ CO2 gasification based chemical looping combustion of low ash coal using Fe2O3 as the oxygen carrier
    Bhui, Barnali
    Vairakannu, Prabu
    JOURNAL OF CO2 UTILIZATION, 2019, 29 : 103 - 116
  • [26] The effects of Na2O/K2O flux on ash fusion characteristics for high silicon-aluminum coal in entrained-flow bed gasification
    Li, Fenghai
    Yang, Ziqiang
    Li, Yang
    Han, Guopeng
    Fan, Hongli
    Liu, Xuefei
    Xu, Meiling
    Guo, Mingxi
    Fang, Yitian
    ENERGY, 2023, 282
  • [27] RECOVERY OF METAL VALUES FROM SPENT COMO/AL2O3 PETROLEUM HYDRODESULFURIZATION AND COAL-LIQUEFACTION CATALYSTS - LABORATORY-SCALE PROCESS AND PRELIMINARY ECONOMICS
    SEBENIK, RF
    FERENCE, RA
    ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 1982, 184 (SEP): : 33 - PETR
  • [28] Attrition of high ash Ekibastuz coal in a bench scale fluidized bed rig under O2/N2 and O2/CO2 environments
    Suleimenova, Botakoz
    Aimbetov, Berik
    Shah, Dhawal
    Anthony, Edward J.
    Sarbassov, Yerbol
    FUEL PROCESSING TECHNOLOGY, 2021, 216
  • [29] Chemical looping based co-combustion of high ash Indian coal and rice straw operating under CO2 in-situ gasification mode
    Bhui, Barnali
    Prabu, V
    JOURNAL OF THE ENERGY INSTITUTE, 2021, 94 : 176 - 190
  • [30] Melting and Flow Behavior of Coal Ash at High Temperatures Based on SiO2-Al2O3-CaO/Na2O Pseudoternary Phase Diagram
    Li, Ping
    Kan, Haoyong
    Chen, Cai
    Wu, Jianjun
    Zhang, Yixin
    Guo, Fanhui
    ACS OMEGA, 2024, 9 (20): : 22313 - 22324