Visible electroluminescence from silicon nanocrystals embedded in amorphous silicon nitride matrix

被引:92
作者
Chen, LY
Chen, WH
Hong, FCN
机构
[1] Natl Cheng Kung Univ, Dept Chem Engn, Tainan 70101, Taiwan
[2] Natl Cheng Kung Univ, Ctr Micro Nano Technol, Tainan 70101, Taiwan
关键词
D O I
10.1063/1.1925311
中图分类号
O59 [应用物理学];
学科分类号
摘要
Visible electroluminescence from silicon nanocrystals (Si-NCs) embedded in amorphous silicon nitride (a-SiNx) films has been observed. The Si-NC/a-SiNx films were deposited by evaporating silicon from electron gun into the inductively coupled plasma of nitrogen. The density of Si-NCs in the a-SiNx matrix was around 10(12) cm(-2). Strong room temperature photoluminescence was observed in 2.8 and 3.0 eV, different from literature values. The electroluminescence (EL) devices were fabricated with Si-NCs/a-SiNx film as the active layer using the Al or Ca/Ag cathode and the indium tin oxide anode. Through tunneling, the electrons and holes were respectively injected from the cathode and anode into Si-NCs and confined within Si-NCs for light emission by the high band gap a-SiNx matrix. For the device with Ca/Ag cathode, the turn-on voltage was as low as 10 V and the EL efficiency was about 1.6 x 10(-1) Cd/A. The EL spectra consisted of two broad peaks centered around 2.5 and 2.8 eV. Our results demonstrate that Si-NCs/a-SiNx nanocomposite films have potentials to be fabricated into electroluminescence devices using the low work function cathode. (c) 2005 American Institute of Physics.
引用
收藏
页码:1 / 3
页数:3
相关论文
共 50 条
[41]   Electroluminescence of single silicon nanocrystals [J].
Valenta, J ;
Lalic, N ;
Linnros, J .
APPLIED PHYSICS LETTERS, 2004, 84 (09) :1459-1461
[42]   Origin of visible luminescence in hydrogenated amorphous silicon nitride [J].
Hao, H. L. ;
Wu, L. K. ;
Shen, W. Z. ;
Dekkers, H. F. W. .
APPLIED PHYSICS LETTERS, 2007, 91 (20)
[43]   Electron charging and discharging in amorphous silicon quantum dots embedded in silicon nitride [J].
Park, NM ;
Choi, SH ;
Park, SJ .
APPLIED PHYSICS LETTERS, 2002, 81 (06) :1092-1094
[44]   Excitonic photoluminescence characteristics of amorphous silicon nanoparticles embedded in silicon nitride film [J].
Yu, W. ;
Zhang, J. Y. ;
Ding, W. G. ;
Fu, G. S. .
EUROPEAN PHYSICAL JOURNAL B, 2007, 57 (01) :53-56
[45]   Excitonic photoluminescence characteristics of amorphous silicon nanoparticles embedded in silicon nitride film [J].
W. Yu ;
J. Y. Zhang ;
W. G. Ding ;
G. S. Fu .
The European Physical Journal B, 2007, 57 :53-56
[46]   Shrinking of silicon nanocrystals embedded in an amorphous silicon oxide matrix during rapid thermal annealing in a forming gas atmosphere [J].
van Sebille, M. ;
Fusi, A. ;
Xie, L. ;
Ali, H. ;
van Swaaij, R. A. C. M. M. ;
Leifer, K. ;
Zeman, M. .
NANOTECHNOLOGY, 2016, 27 (36)
[47]   Optical spectra of crystalline silicon particles embedded in an amorphous silicon matrix [J].
Kwon, D ;
Lee, H ;
Cohen, JD ;
Jin, HC ;
Abelson, JR .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 1998, 227 :1040-1044
[48]   Optical spectra of crystalline silicon particles embedded in an amorphous silicon matrix [J].
Univ of Oregon, Eugene, United States .
J Non Cryst Solids, Pt 2 (1040-1044)
[49]   Photocurrent and Photoluminescence of Amorphous Silicon Nanoclusters Embedded in Silicon Suboxide Matrix [J].
Sreseli, O. M. ;
Gusev, O. B. ;
Vainshtein, J. S. ;
Undalov, Yu K. ;
Yeltsina, O. S. ;
Sitnikova, A. A. ;
Terukov, E. I. .
GETTERING AND DEFECT ENGINEERING IN SEMICONDUCTOR TECHNOLOGY XIV, 2011, 178-179 :465-470
[50]   Electroluminescence from silicon-rich nitride/silicon superlattice structures [J].
Warga, J. ;
Li, R. ;
Basu, S. N. ;
Dal Negro, L. .
APPLIED PHYSICS LETTERS, 2008, 93 (15)