Concentrations, Source Identification, and Lung Cancer Risk Associated with Springtime PM2.5-Bound Polycyclic Aromatic Hydrocarbons (PAHs) in Nanjing, China

被引:25
作者
Chen, Chong [1 ,2 ]
Xia, Zhonghuan [1 ,2 ,3 ,4 ]
Wu, Minmin [1 ,2 ]
Zhang, Qianqian [1 ,2 ]
Wang, Tao [1 ,2 ]
Wang, Liping [1 ,2 ]
Yang, Hao [2 ,3 ,4 ]
机构
[1] Nanjing Normal Univ, Jiangsu Prov Key Lab Mat Cycling & Pollut Control, Sch Environm, Nanjing 210023, Jiangsu, Peoples R China
[2] Nanjing Normal Univ, Key Lab Virtual Geog Environm, Minist Educ, Nanjing 210023, Jiangsu, Peoples R China
[3] Jiangsu Ctr Collaborat Innovat Geog Informat Reso, Nanjing 210023, Jiangsu, Peoples R China
[4] State Key Lab Cultivat Base Geog Environm Evolut, Nanjing 210023, Jiangsu, Peoples R China
基金
中国国家自然科学基金; 中国博士后科学基金;
关键词
MOLECULAR DIAGNOSTIC RATIOS; SOURCE APPORTIONMENT; URBAN; PARTICULATE; EXPOSURE; AREAS; PM2.5; CITY;
D O I
10.1007/s00244-017-0435-4
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study concentrated on the pollution level, sources, and lung cancer risk of PM2.5-bound polycyclic aromatic hydrocarbons (PAHs) in spring in Nanjing, China. The PM2.5 samples were collected in spring of the year 2016 in Nanjing. Sixteen United States Environmental Protection Agency priority PAHs were extracted and analyzed after sampling. The mean concentrations of PAHs and BaPeq were 3.98 +/- 1.01 and 0.29 +/- 0.08 ng/m(3), respectively, which is a low level among results from regions worldwide. The diurnal variations of PAHs and BaPeq concentrations showed a relatively high level in the early morning, at the morning rush time of work and traffic transportation, and in the evening traffic peak hours. According to the results of diagnostic ratios, PAHs originated mainly from traffic exhaust, especially diesel vehicle emissions. In a single day, the highest inhalation exposure level was focused between 4 a.m. and 6 a.m., whereas the time between 12 a.m. to 2 p.m. in a day had the lowest exposure dose. Due to the inhalation exposure, the median values of incremental lung cancer risk in spring were estimated to be 7.08 x 10(-9), 5.29 x 10(-9), 3.53 x 10(-8), 5.21 x 10(-9), 7.21 x 10(-9), 5.24 x 10(-9), 3.01 x 10(-8), and 5.40 x 10(-9) for boys, male adolescents, male adults, male seniors, girls, female adolescents, female adults, and female seniors, respectively, indicating low potential lung cancer risk.
引用
收藏
页码:391 / 400
页数:10
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