Methane emissions: choosing the right climate metric and time horizon

被引:137
作者
Balcombe, Paul [1 ,2 ]
Speirs, Jamie F. [2 ,3 ]
Brandon, Nigel P. [2 ,3 ]
Hawkes, Adam D. [1 ,2 ]
机构
[1] Imperial Coll London, Dept Chem Engn, London SW7 2AZ, England
[2] Imperial Coll London, Sustainable Gas Inst, London SW7 1NA, England
[3] Imperial Coll London, Dept Earth Sci & Engn, London SW7 2BP, England
基金
巴西圣保罗研究基金会;
关键词
GLOBAL WARMING POTENTIALS; CYCLE IMPACT ASSESSMENT; LIQUEFIED NATURAL-GAS; CARBON-DIOXIDE; TRADE-OFFS; POLICY; AEROSOLS; LNG;
D O I
10.1039/c8em00414e
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Methane is a more potent greenhouse gas (GHG) than CO2, but it has a shorter atmospheric lifespan, thus its relative climate impact reduces significantly over time. Different GHGs are often conflated into a single metric to compare technologies and supply chains, such as the global warming potential (GWP). However, the use of GWP is criticised, regarding: (1) the need to select a timeframe; (2) its physical basis on radiative forcing; and (3) the fact that it measures the average forcing of a pulse over time rather than a sustained emission at a specific end-point in time. Many alternative metrics have been proposed which tackle different aspects of these limitations and this paper assesses them by their key attributes and limitations, with respect to methane emissions. A case study application of various metrics is produced and recommendations are made for the use of climate metrics for different categories of applications. Across metrics, CO2 equivalences for methane range from 4-199 gCO(2eq.)/gCH(4), although most estimates fall between 20 and 80 gCO(2eq.)/gCH(4). Therefore the selection of metric and time horizon for technology evaluations is likely to change the rank order of preference, as demonstrated herein with the use of natural gas as a shipping fuel versus alternatives. It is not advisable or conservative to use only a short time horizon, e.g. 20 years, which disregards the long-term impacts of CO2 emissions and is thus detrimental to achieving eventual climate stabilisation. Recommendations are made for the use of metrics in 3 categories of applications. Short-term emissions estimates of facilities or regions should be transparent and use a single metric and include the separated contribution from each GHG. Multi-year technology assessments should use both short and long term static metrics (e.g. GWP) to test robustness of results. Longer term energy assessments or decarbonisation pathways must use both short and long-term metrics and where this has a large impact on results, climate models should be incorporated. Dynamic metrics offer insight into the timing of emissions, but may be of only marginal benefit given uncertainties in methodological assumptions.
引用
收藏
页码:1323 / 1339
页数:17
相关论文
共 66 条
[31]   Assessment of full life-cycle air emissions of alternative shipping fuels [J].
Gilbert, Paul ;
Walsh, Conor ;
Traut, Michael ;
Kesieme, Uchenna ;
Pazouki, Kayvan ;
Murphy, Alan .
JOURNAL OF CLEANER PRODUCTION, 2018, 172 :855-866
[32]   Estimates of the direct and indirect radiative forcing due to tropospheric aerosols: A review [J].
Haywood, J ;
Boucher, O .
REVIEWS OF GEOPHYSICS, 2000, 38 (04) :513-543
[33]   Life cycle GHG emission analysis of power generation systems: Japanese case [J].
Hondo, H .
ENERGY, 2005, 30 (11-12) :2042-2056
[34]   Methane and the greenhouse-gas footprint of natural gas from shale formations [J].
Howarth, Robert W. ;
Santoro, Renee ;
Ingraffea, Anthony .
CLIMATIC CHANGE, 2011, 106 (04) :679-690
[35]   The implications of carbon dioxide and methane exchange for the heavy mitigation RCP2.6 scenario under two metrics [J].
Huntingford, Chris ;
Lowe, Jason A. ;
Howarth, Nicholas ;
Bowerman, Niel H. A. ;
Gohar, Laila K. ;
Otto, Alexander ;
Lee, David S. ;
Smith, Stephen M. ;
den Elzen, Michel G. J. ;
van Vuuren, Detlef P. ;
Millar, Richard J. ;
Allen, Myles R. .
ENVIRONMENTAL SCIENCE & POLICY, 2015, 51 :77-87
[36]  
IEA, 2017, WORLD EN OUTL 2017
[37]   Economics- and physical-based metrics for comparing greenhouse gases [J].
Johansson, Daniel J. A. .
CLIMATIC CHANGE, 2012, 110 (1-2) :123-141
[38]   THE RELATIVE ROLE OF TRACE GAS EMISSIONS IN GREENHOUSE ABATEMENT POLICIES [J].
KANDLIKAR, M .
ENERGY POLICY, 1995, 23 (10) :879-883
[39]   Climate-change impact potentials as an alternative to global warming potentials [J].
Kirschbaum, Miko U. F. .
ENVIRONMENTAL RESEARCH LETTERS, 2014, 9 (03)
[40]   Global Carbon Budget 2016 [J].
Le Quere, Corinne ;
Andrew, Robbie M. ;
Canadell, Josep G. ;
Sitch, Stephen ;
Korsbakken, Jan Ivar ;
Peters, Glen P. ;
Manning, Andrew C. ;
Boden, Thomas A. ;
Tans, Pieter P. ;
Houghton, Richard A. ;
Keeling, Ralph F. ;
Alin, Simone ;
Andrews, Oliver D. ;
Anthoni, Peter ;
Barbero, Leticia ;
Bopp, Laurent ;
Chevallier, Frederic ;
Chini, Louise P. ;
Ciais, Philippe ;
Currie, Kim ;
Delire, Christine ;
Doney, Scott C. ;
Friedlingstein, Pierre ;
Gkritzalis, Thanos ;
Harris, Ian ;
Hauck, Judith ;
Haverd, Vanessa ;
Hoppema, Mario ;
Goldewijk, Kees Klein ;
Jain, Atul K. ;
Kato, Etsushi ;
Koertzinger, Arne ;
Landschuetzer, Peter ;
Lefevre, Nathalie ;
Lenton, Andrew ;
Lienert, Sebastian ;
Lombardozzi, Danica ;
Melton, Joe R. ;
Metzl, Nicolas ;
Millero, Frank ;
Monteiro, Pedro M. S. ;
Munro, David R. ;
Nabel, Julia E. M. S. ;
Nakaoka, Shin-ichiro ;
O'Brien, Kevin ;
Olsen, Are ;
Omar, Abdirahman M. ;
Ono, Tsuneo ;
Pierrot, Denis ;
Poulter, Benjamin .
EARTH SYSTEM SCIENCE DATA, 2016, 8 (02) :605-649