One-pot imine synthesis from methylarenes and anilines under air over heterogeneous Cu oxide-modified CeO2catalyst

被引:6
|
作者
Tamura, Masazumi [1 ]
Li, Yingai [2 ]
Tomishige, Keiichi [2 ]
机构
[1] Osaka City Univ, Adv Res Inst Nat Sci & Technol, Res Ctr Artificial Photosynth, Sumiyoshi Ku, 3-3-138 Sugimoto, Osaka 5588585, Japan
[2] Tohoku Univ, Sch Engn, Dept Appl Chem, Aoba Ku, 6-6-07 Aoba, Sendai, Miyagi 9808579, Japan
关键词
CARBONYL-COMPOUNDS; DIRECT AMIDATION; CEO2; OXIDATION; CATALYST; OXYGEN; EFFICIENT; BENZIMIDAZOLES; HYDROGENATION; NITROARENES;
D O I
10.1039/d0cc02969f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Cu oxide-modified CeO2(CuOx-CeO2) with 2 wt% Cu loading amount was the most effective and reusable heterogeneous catalyst for selective one-pot imine synthesis from methylarenes and anilinesviadirect oxidation of the sp(3)C-H bond in the methylarenes with atmospheric air (0.1 MPa) as an oxidant.
引用
收藏
页码:7337 / 7340
页数:4
相关论文
共 26 条
  • [1] Hydrotalcite-Supported Ceria Nanoparticles as a Heterogeneous Catalyst for One-Pot Synthesis of Imines under Atmospheric Air
    Tomar, Ravi
    Ebitani, Kohki
    Chandra, Ramesh
    CHEMISTRYSELECT, 2019, 4 (12): : 3577 - 3581
  • [2] CO2 Recycling into CH4 and H2O over Ru/CeO2 Catalyst Prepared by one-pot Synthesis
    Tuti, Simonetta
    Laverdura, Umberto Pasqual
    Luisetto, Igor
    Lo Mastro, Sergio
    Stendardo, Stefano
    2022 IEEE INTERNATIONAL WORKSHOP ON METROLOGY FOR AEROSPACE (IEEE METROAEROSPACE 2022), 2022, : 390 - 395
  • [3] One-Pot Synthesis of Styrene Carbonate from Styrene and CO2 Over the Nanogold-Ionic Liquid Catalyst
    Jasiak, Katarzyna
    Krawczyk, Tomasz
    Pawlyta, Miroslawa
    Jakobik-Kolon, Agata
    Baj, Stefan
    CATALYSIS LETTERS, 2016, 146 (05) : 893 - 901
  • [4] One-Pot Synthesis of Cu-SO42--ZrO2 Catalysts for Use as Acid Catalyst in Dimethyl Ether Production from CO2 Hydrogenation
    Numpilai, Thanapha
    Dolsiririttigul, Napaphut
    Laobuthee, Apirat
    Cheng, Chin Kui
    Chanlek, Narong
    Poo-arporn, Yingyot
    Witoon, Thongthai
    TOPICS IN CATALYSIS, 2023, 66 (19-20) : 1467 - 1477
  • [5] CeO2 immobilized on magnetic core-shell microparticles for one-pot synthesis of imines from benzyl alcohols and anilines: Support effects for activity and stability
    Long, Yu
    Gao, Zekun
    Qin, Jiaheng
    Wang, Peng
    Wu, Wei
    Zhang, Lin
    Dong, Zhengping
    Ma, Jiantai
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2019, 538 : 709 - 719
  • [6] One-pot synthesis of alanine from glycerol without additional H2 over a rutile-supported Ru catalyst
    Li, Jiachen
    Tang, Zhenchen
    Ahmadi, Majid
    Yang, Huaizhou
    Gerlach, Dominic
    Kooi, Bart J.
    Rudolf, Petra
    Heeres, Hero J.
    Pescarmona, Paolo P.
    APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY, 2025, 365
  • [7] A protective roasting strategy for preparation of stable mesoporous hollow CeO2 microspheres with enhanced catalytic activity for one-pot synthesis of imines from benzyl alcohols and anilines
    Long, Yu
    Zhang, Hongbo
    Gao, Zekun
    Qin, Jiaheng
    Pan, Yiting
    Zhao, Jinping
    Luo, Yutong
    Ma, Zhiping
    Xiong, Yucong
    Ma, Jiantai
    INORGANIC CHEMISTRY FRONTIERS, 2019, 6 (03) : 829 - 836
  • [8] One-pot synthesis of benzoazoles via dehydrogenative coupling of aromatic 1,2-diamines/2-aminothiophenol and alcohols using Pd/Cu-MOF as a recyclable heterogeneous catalyst
    Mokhtari, Javad
    Bozcheloei, Abolfazl Hasani
    INORGANICA CHIMICA ACTA, 2018, 482 : 726 - 731
  • [9] Synthesis of FAU Zeolite Nanoparticles as Heterogeneous Catalyst for One-Pot Synthesis of 2-Substituted Aryl (Indolyl) Kojic Acid Derivatives under Solvent-Free Condition
    Sadeghi, Bahareh
    Lasemi, Zahra
    Tavasoli, Fereshteh Amiri
    Hashemian, Saeedeh
    Zahedi, Hesam
    SYNTHESIS AND REACTIVITY IN INORGANIC METAL-ORGANIC AND NANO-METAL CHEMISTRY, 2014, 44 (10) : 1497 - 1503
  • [10] Heterogeneously Catalyzed One-Pot Synthesis of N-alkyl Anilines from Nitroaromatics by Assembled Pt3Sn/Al2O3 Catalyst
    Yang Fang
    Xu Xiang-Sheng
    Gu Hui-Zi
    Chen Ao-Ang
    Yan Xin-Huan
    ACTA PHYSICO-CHIMICA SINICA, 2012, 28 (09) : 2141 - 2147