Diagnostic studies of ac-driven plasmas in saline solutions: the effect of frequency on the plasma behavior

被引:17
作者
Chang, Hung-wen [1 ]
Hsu, Cheng-che [1 ]
机构
[1] Natl Taiwan Univ, Dept Chem Engn, Taipei 10764, Taiwan
关键词
DISCHARGE; WATER; CONTACT; CHEMISTRY; BUBBLES; PHYSICS; VAPOR; FLOW;
D O I
10.1088/0963-0252/20/4/045001
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
The effect of frequency on the characteristics of plasmas in saline solution driven by 50-1000 Hz ac power is studied. Two distinct modes, namely bubble and jetting modes, are identified. The bubble mode occurs under low frequencies. In this mode, a millimeter-sized bubble is tightly attached to the electrode tip and oscillates with the applied voltage. With an increase in frequency, it shows the jetting mode, in which bubbles, hundreds of micometers in diameter, are continuously formed and jetted away from the electrode surface. Such a significant change in the bubble behavior influences the power input at a given applied voltage and significantly affects the plasma behavior. In spite of the fact that no significant difference is seen in the optical emission spectra, the broadening of the H-beta peak shows that the bubble mode has a lower electron density than that of the jetting mode. The temporally resolved optical emission intensities show light emission in the negative half of the power period regardless of the modes. This shows clearly that the driving frequency significantly influences the bubble dynamics, which in turn alters the plasma behavior.
引用
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页数:9
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共 39 条
[1]   Self-pulsing regime of DC electric discharge in dielectric tube filled with water containing gas bubble [J].
Akishev, Yuri ;
Grushin, Michail ;
Karalnik, Vlad ;
Monich, Anton ;
Petryakov, Alex ;
Trushkin, Nikolay .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 2008, 36 (04) :1142-1143
[2]   Mechanism of spark generation during electrochemical discharge machining: A theoretical model and experimental verification [J].
Basak, I ;
Ghosh, A .
JOURNAL OF MATERIALS PROCESSING TECHNOLOGY, 1996, 62 (1-3) :46-53
[3]   Localized Synthesis of Metal Nanoparticles Using Nanoscale Corona Discharge in Aqueous Solutions [J].
Bhattacharyya, Sayan ;
Staack, David ;
Vitol, Elina A. ;
Singhal, Riju ;
Fridman, Alexander ;
Friedman, Gary ;
Gogotsi, Yury .
ADVANCED MATERIALS, 2009, 21 (40) :4039-+
[4]   Experimental investigation of dc electrical breakdown of long vapour bubbles in capillaries [J].
Bruggeman, Peter ;
Leys, Christophe ;
Vierendeels, Jan .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2007, 40 (07) :1937-1943
[5]   DC-excited discharges in vapour bubbles in capillaries [J].
Bruggeman, Peter ;
Degroote, Joris ;
Vierendeels, Jan ;
Leys, Christophe .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 2008, 17 (02)
[6]   Characterization of a direct dc-excited discharge in water by optical emission spectroscopy [J].
Bruggeman, Peter ;
Schram, Daan ;
Gonzalez, Manuel A. ;
Rego, Robby ;
Kong, Michael G. ;
Leys, Christophe .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 2009, 18 (02)
[7]   PRELIMINARY INVESTIGATION OF PREBREAKDOWN PHENOMENA AND CHEMICAL-REACTIONS USING A PULSED HIGH-VOLTAGE DISCHARGE IN WATER [J].
CLEMENTS, JS ;
SATO, M ;
DAVIS, RH .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1987, 23 (02) :224-235
[8]   DIFFUSION AND ATTACHMENT OF ELECTRONS IN WATER VAPOUR [J].
CROMPTON, RW ;
REES, JA ;
JORY, RL .
AUSTRALIAN JOURNAL OF PHYSICS, 1965, 18 (06) :541-&
[9]   Basics of plasma spectroscopy [J].
Fantz, U. .
PLASMA SOURCES SCIENCE & TECHNOLOGY, 2006, 15 (04) :S137-S147
[10]   Spark assisted chemical engraving in the light of electrochemistry [J].
Fascio, V ;
Wüthrich, R ;
Bleuler, H .
ELECTROCHIMICA ACTA, 2004, 49 (22-23) :3997-4003