A new regime of nanoscale thermal transport: Collective diffusion increases dissipation efficiency

被引:156
作者
Hoogeboom-Pot, Kathleen M. [1 ,2 ]
Hernandez-Charpak, Jorge N. [1 ,2 ]
Gu, Xiaokun [3 ]
Frazer, Travis D. [1 ,2 ]
Anderson, Erik H. [4 ]
Chao, Weilun [4 ]
Falcone, Roger W. [4 ]
Yang, Ronggui [3 ]
Murnane, Margaret M. [1 ,2 ]
Kapteyn, Henry C. [1 ,2 ]
Nardi, Damiano [1 ,2 ]
机构
[1] Univ Colorado, JILA, Boulder, CO 80309 USA
[2] Univ Colorado, Dept Phys, Boulder, CO 80309 USA
[3] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA
[4] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA
基金
美国国家科学基金会;
关键词
nanoscale thermal transport; nondiffusive transport; mean free path spectroscopy; high harmonic generation; ultrafast X-rays; GENERATION;
D O I
10.1073/pnas.1503449112
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Understanding thermal transport from nanoscale heat sources is important for a fundamental description of energy flow in materials, as well as for many technological applications including thermal management in nanoelectronics and optoelectronics, thermoelectric devices, nanoenhanced photovoltaics, and nanoparticle-mediated thermal therapies. Thermal transport at the nanoscale is fundamentally different from that at the macroscale and is determined by the distribution of carrier mean free paths and energy dispersion in a material, the length scales of the heat sources, and the distance over which heat is transported. Past work has shown that Fourier's law for heat conduction dramatically overpredicts the rate of heat dissipation from heat sources with dimensions smaller than the mean free path of the dominant heat-carrying phonons. In this work, we uncover a new regime of nanoscale thermal transport that dominates when the separation between nanoscale heat sources is small compared with the dominant phononmean free paths. Surprisingly, the interaction of phonons originating from neighboring heat sources enables more efficient diffusive-like heat dissipation, even from nanoscale heat sources much smaller than the dominant phonon mean free paths. This finding suggests that thermal management in nanoscale systems including integrated circuits might not be as challenging as previously projected. Finally, we demonstrate a unique capability to extract differential conductivity as a function of phonon mean free path in materials, allowing the first ( to our knowledge) experimental validation of predictions from the recently developed first-principles calculations.
引用
收藏
页码:4846 / 4851
页数:6
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