Water distribution measurement for a PEMFC through neutron radiography

被引:84
作者
Chen, Yong-Song
Peng, Huei
Hussey, Daniel S.
Jacobson, David L.
tran, Doanh T.
Abdel-Baset, Tarek
Biernacki, Mark
机构
[1] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA
[2] Natl Inst Stand & Technol, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[3] DaimlerChrysler Corp, Auburn Hills, MI 48326 USA
基金
美国国家科学基金会;
关键词
PEMFC; water visualization; water management; neutron radiography;
D O I
10.1016/j.jpowsour.2007.03.076
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Neutron radiography has been used for in situ and non-destructive visualization and measurement technique for liquid water in a working proton-exchange membrane fuel cell (PEMFC). In an attempt to differentiate water distribution in the anode side from that in the cathode side, a specially designed cell was machined and used for the experiment. The major difference between our design and traditional flow field design is the fact the anode channels and cathode channels were shifted by a channel width, so that the anode and cathode channels do not overlap in the majority of the active areas. The neutron radiography experiments were performed at selected relative humidities, and stoichiometry values of cathode inlet. At each operating condition, the water distribution in anode/cathode gas diffusion layers (GDLs) was obtained. Image processing with four different spatial masks was applied to those images to differentiate liquid water in four different types of areas. Results indicate that the reactant gas relative humidity and stoichiometry significantly influence current density distribution and water distribution. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:376 / 386
页数:11
相关论文
共 18 条
[11]   Study of water distribution and transport in a polymer electrolyte fuel cell using neutron imaging [J].
Pekula, N ;
Heller, K ;
Chuang, PA ;
Turhan, A ;
Mench, MM ;
Brenizer, JS ;
Ünlü, K .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2005, 542 (1-3) :134-141
[12]   In situ neutron imaging technique for evaluation of water management systems in operating PEM fuel cells [J].
Satija, R ;
Jacobson, DL ;
Arif, M ;
Werner, SA .
JOURNAL OF POWER SOURCES, 2004, 129 (02) :238-245
[13]   Spatially resolved characterization of PEFCs using simultaneously neutron radiography and locally resolved impedance spectroscopy [J].
Schneider, IA ;
Kramer, D ;
Wokaun, A ;
Scherer, GG .
ELECTROCHEMISTRY COMMUNICATIONS, 2005, 7 (12) :1393-1397
[14]   Visualization of water buildup in the cathode of a transparent PEM fuel cell [J].
Tüber, K ;
Pócza, D ;
Hebling, C .
JOURNAL OF POWER SOURCES, 2003, 124 (02) :403-414
[15]   Quantification of liquid water accumulation and distribution in a polymer electrolyte fuel cell using neutron imaging [J].
Turhan, A. ;
Heller, K. ;
Brenizer, J. S. ;
Mench, M. M. .
JOURNAL OF POWER SOURCES, 2006, 160 (02) :1195-1203
[16]   Two-phase flow and transport in the air cathode of proton exchange membrane fuel cells [J].
Wang, ZH ;
Wang, CY ;
Chen, KS .
JOURNAL OF POWER SOURCES, 2001, 94 (01) :40-50
[17]   THE WATER-CONTENT DEPENDENCE OF ELECTROOSMOTIC DRAG IN PROTON-CONDUCTING POLYMER ELECTROLYTES [J].
ZAWODZINSKI, TA ;
DAVEY, J ;
VALERIO, J ;
GOTTESFELD, S .
ELECTROCHIMICA ACTA, 1995, 40 (03) :297-302
[18]   In situ diagnostic of two-phase flow phenomena in polymer electrolyte fuel cells by neutron imaging Part B. Material variations [J].
Zhang, JB ;
Kramer, D ;
Shimoi, R ;
Ona, Y ;
Lehmann, E ;
Wokaun, A ;
Shinohara, K ;
Scherer, GG .
ELECTROCHIMICA ACTA, 2006, 51 (13) :2715-2727