PEMFC;
water visualization;
water management;
neutron radiography;
D O I:
10.1016/j.jpowsour.2007.03.076
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Neutron radiography has been used for in situ and non-destructive visualization and measurement technique for liquid water in a working proton-exchange membrane fuel cell (PEMFC). In an attempt to differentiate water distribution in the anode side from that in the cathode side, a specially designed cell was machined and used for the experiment. The major difference between our design and traditional flow field design is the fact the anode channels and cathode channels were shifted by a channel width, so that the anode and cathode channels do not overlap in the majority of the active areas. The neutron radiography experiments were performed at selected relative humidities, and stoichiometry values of cathode inlet. At each operating condition, the water distribution in anode/cathode gas diffusion layers (GDLs) was obtained. Image processing with four different spatial masks was applied to those images to differentiate liquid water in four different types of areas. Results indicate that the reactant gas relative humidity and stoichiometry significantly influence current density distribution and water distribution. (c) 2007 Elsevier B.V. All rights reserved.
机构:
Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Kramer, D
;
Zhang, JB
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机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Zhang, JB
;
Shimoi, R
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机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shimoi, R
;
Lehmann, E
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机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Lehmann, E
;
Wokaun, A
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机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Wokaun, A
;
Shinohara, K
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机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shinohara, K
;
Scherer, GG
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机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
机构:
Penn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Mench, MM
;
Dong, QL
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机构:
Penn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Dong, QL
;
Wang, CY
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
机构:
Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, SwitzerlandPaul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Kramer, D
;
Zhang, JB
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Zhang, JB
;
Shimoi, R
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shimoi, R
;
Lehmann, E
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Lehmann, E
;
Wokaun, A
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Wokaun, A
;
Shinohara, K
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
Shinohara, K
;
Scherer, GG
论文数: 0引用数: 0
h-index: 0
机构:Paul Scherrer Inst, Gen Energy Dept, Electrochem Lab, CH-5232 Villigen, Switzerland
机构:
Penn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Mench, MM
;
Dong, QL
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USA
Dong, QL
;
Wang, CY
论文数: 0引用数: 0
h-index: 0
机构:
Penn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USAPenn State Univ, Electrochem Engine Ctr, Dept Mech & Nucl Engn, University Pk, PA 16802 USA