Wearable, Washable, and Highly Sensitive Piezoresistive Pressure Sensor Based on a 3D Sponge Network for Real-Time Monitoring Human Body Activities

被引:91
作者
Li, Xiaodi [1 ,2 ]
Li, Xu [1 ]
Liu, Ting [1 ]
Lu, Yong [1 ]
Shang, Chengshuo [3 ,4 ]
Ding, Xiaokang [2 ,3 ,4 ]
Zhang, Jicai [1 ,3 ,4 ]
Feng, Yongjun [2 ]
Xu, Fu-Jian [2 ,3 ,4 ]
机构
[1] Beijing Univ Chem Technol, Coll Math & Phys, Beijing 100029, Peoples R China
[2] Beijing Univ Chem Technol, State Key Lab Chem Resource Engn, Beijing 100029, Peoples R China
[3] Beijing Univ Chem Technol, Minist Educ, Lab Biomed Mat, Beijing 100029, Peoples R China
[4] Beijing Univ Chem Technol, Minist Educ, Key Lab Biomed Mat Nat Macromol, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
MXene; sponge; piezoresistive sensor; wearable; washable; COMPOSITES;
D O I
10.1021/acsami.1c09975
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Wearable pressure sensors are highly desirable for monitoring human health and realizing a nice human-machine interaction. Herein, a chitosan/MXene/polyurethane-sponge/polyvinyl alcohol (CS/MXene/PU sponge/PVA)-based 3D pressure sensor is developed to simultaneously achieve wearability, washability, and high sensitivity in a wide region. In the force-sensitive layer of the sensor, MXene and CS are fully attached to the PU sponge to ensure that the composite sponge has remarkable conductivity and washability. Benefiting from the highly resistive PVA-nanowire spacer, the initial current of the sensor is reduced significantly so that the sensor exhibits extremely high sensitivity (84.9 kPa(-1) for the less than 5 kPa region and 140.6 kPa(-1) for the 5-22 kPa region). Moreover, the sensor has an excellent fast response time of 200 ms and a short recovery time of 30 ms, as well as non-attenuating durability over 5000 cycles. With the high sensitivity in a wide range, the sensor is capable of detecting multiple human and animal activities in real time, ranging from the large pressure of joint activities to a subtle pressure of pulse. Furthermore, the sensor also demonstrates the potential application in measuring pressure distribution. Overall, such a multifunctional pressure sensor can supply a new platform for the design and development of wearable health-monitoring equipment and an efficient human-machine interface.
引用
收藏
页码:46848 / 46857
页数:10
相关论文
共 51 条
[1]   Engineered Exosome-Mediated Near-Infrared-II Region V2C Quantum Dot Delivery for Nucleus-Target Low-Temperature Photothermal Therapy [J].
Cao, Yu ;
Wu, Tingting ;
Zhang, Kai ;
Meng, Xiangdan ;
Dai, Wenhao ;
Wang, Dongdong ;
Dong, Haifeng ;
Zhang, Xueji .
ACS NANO, 2019, 13 (02) :1499-1510
[2]   Flexible Piezoelectric-Induced Pressure Sensors for Static Measurements Based on Nanowires/Graphene Heterostructures [J].
Chen, Zefeng ;
Wang, Zhao ;
Li, Xinming ;
Lin, Yuxuan ;
Luo, Ningqi ;
Long, Mingzhu ;
Zhao, Ni ;
Xu, Jian-Bin .
ACS NANO, 2017, 11 (05) :4507-4513
[3]   Compressible, Elastic, and Pressure-Sensitive Carbon Aerogels Derived from 2D Titanium Carbide Nanosheets and Bacterial Cellulose for Wearable Sensors [J].
Chen, Zehong ;
Hu, Yijie ;
Zhuo, Hao ;
Liu, Linxiang ;
Jing, Shuangshuang ;
Zhong, Linxin ;
Peng, Xinwen ;
Sun, Run-cang .
CHEMISTRY OF MATERIALS, 2019, 31 (09) :3301-3312
[4]   Lightweight and Flexible Graphene Foam Composites for High-Performance Electromagnetic Interference Shielding [J].
Chen, Zongping ;
Xu, Chuan ;
Ma, Chaoqun ;
Ren, Wencai ;
Cheng, Hui-Ming .
ADVANCED MATERIALS, 2013, 25 (09) :1296-1300
[5]   Bioinspired Microspines for a High-Performance Spray Ti3C2Tx MXene-Based Piezoresistive Sensor [J].
Cheng, Yongfa ;
Ma, Yanan ;
Li, Luying ;
Zhu, Meng ;
Yue, Yang ;
Liu, Weijie ;
Wang, Longfei ;
Jia, Shuangfeng ;
Li, Chen ;
Qi, Tianyu ;
Wang, Jianbo ;
Gao, Yihua .
ACS NANO, 2020, 14 (02) :2145-2155
[6]   Wearable and Implantable Soft Bioelectronics Using Two-Dimensional Materials [J].
Choi, Changsoon ;
Lee, Youngsik ;
Cho, Kyoung Won ;
Koo, Ja Hoon ;
Kim, Dae-Hyeong .
ACCOUNTS OF CHEMICAL RESEARCH, 2019, 52 (01) :73-81
[7]   Embossed Hollow Hemisphere-Based Piezoelectric Nanogenerator and Highly Responsive Pressure Sensor [J].
Chun, Jinsung ;
Lee, Keun Young ;
Kang, Chong-Yun ;
Kim, Myung Wha ;
Kim, Sang-Woo ;
Baik, Jeong Min .
ADVANCED FUNCTIONAL MATERIALS, 2014, 24 (14) :2038-2043
[8]   Highly Conductive Optical Quality Solution-Processed Films of 2D Titanium Carbide [J].
Dillon, Andrew D. ;
Ghidiu, Michael J. ;
Krick, Alex L. ;
Griggs, Justin ;
May, Steven J. ;
Gogotsi, Yury ;
Barsoum, Michel W. ;
Fafarman, Aaron T. .
ADVANCED FUNCTIONAL MATERIALS, 2016, 26 (23) :4162-4168
[9]   Microchannel-Confined MXene Based Flexible Piezoresistive Multifunctional Micro-Force Sensor [J].
Gao, Yuyu ;
Yan, Cheng ;
Huang, Haichao ;
Yang, Tao ;
Tian, Guo ;
Xiong, Da ;
Chen, Ningjun ;
Chu, Xiang ;
Zhong, Shen ;
Deng, Weili ;
Fang, Yong ;
Yang, Weiqing .
ADVANCED FUNCTIONAL MATERIALS, 2020, 30 (11)
[10]   Conductive two-dimensional titanium carbide 'clay' with high volumetric capacitance [J].
Ghidiu, Michael ;
Lukatskaya, Maria R. ;
Zhao, Meng-Qiang ;
Gogotsi, Yury ;
Barsoum, Michel W. .
NATURE, 2014, 516 (7529) :78-U171