Indoor polybrominated diphenyl ethers in urban China: An exposure and risk assessment based on settled dust from selected urban regions

被引:15
作者
Bu, Zhongming [1 ]
Xu, Xiaoxue [2 ]
Xu, Qi [1 ]
Mmereki, Daniel [3 ]
Wang, Jiahui [4 ]
Cheng, Zhu [5 ]
Li, Ke [1 ]
Dong, Cong [1 ]
机构
[1] Zhejiang Univ Sci & Technol, Dept Energy & Environm Syst Engn, Hangzhou 310023, Peoples R China
[2] Hangzhou Architectural & Civil Engn Design Inst C, Hangzhou 310020, Peoples R China
[3] Univ Witwatersrand, Sch Publ Hlth, Occupat Hlth Div, Parktown Educ Campus, ZA-2193 Johannesburg, South Africa
[4] Hangzhou Polytech, Inst Urban Construct, Hangzhou 311402, Peoples R China
[5] Sichuan Univ, Coll Architecture & Environm, Chengdu 610065, Peoples R China
基金
中国国家自然科学基金;
关键词
Indoor; Polybrominated diphenyl ethers (PBDEs); Settled dust; Exposure; Health risk; Urban China; BROMINATED FLAME-RETARDANTS; PERSISTENT ORGANIC POLLUTANTS; HAZARDOUS AIR-POLLUTANTS; IN-HOUSE DUST; HEALTH-RISK; POLYCHLORINATED-BIPHENYLS; INHALATION EXPOSURE; PHTHALATE EXPOSURE; PARTICLE-SIZE; PBDES;
D O I
10.1016/j.scitotenv.2020.136808
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this study, measurements of seven typical polybrominated diphenyl ethers (PBDEs) in indoor settled dust were summarized in selected urban regions of China. BDE-209 was the most dominant congener in settled dust (1.4-101 mu g/g), with a mean contribution of 95%. Indoor exposures to PBDEs were estimated via inhalation, dust ingestion, and dermal absorption. The average daily intake of Sigma PBDE was 4.9 to 19.1 ng/day/kg for all the population groups, with >80% of the total exposures from dust ingestion. Exposures in commuting environments (contributing 60%-80% of the total exposures) were higher than those in other microenvironments.The means of hazard indexes ranged from 1.66 x 10(-3) to 526 x 10(-3), which were mainly as a result of exposure to BDE-209, BDE-47, and BDE-99.The average lifetime cancer risks were from 0.03 x 10(-9) to 2.37 x 10(-9), which indicated the acceptable health risks resulting from indoor PBDE exposure for the Chinese population.The present study could provide valuable information that could be helpful for decision-makers, analysts and researchers to develop, implement and evaluate the effectiveness of interventions for the reduction of exposures to semi-volatile organic compounds (SVOCs) for large population groups in China. (C) 2020 Published by Elsevier B.V.
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页数:10
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