Indoor polybrominated diphenyl ethers in urban China: An exposure and risk assessment based on settled dust from selected urban regions

被引:15
作者
Bu, Zhongming [1 ]
Xu, Xiaoxue [2 ]
Xu, Qi [1 ]
Mmereki, Daniel [3 ]
Wang, Jiahui [4 ]
Cheng, Zhu [5 ]
Li, Ke [1 ]
Dong, Cong [1 ]
机构
[1] Zhejiang Univ Sci & Technol, Dept Energy & Environm Syst Engn, Hangzhou 310023, Peoples R China
[2] Hangzhou Architectural & Civil Engn Design Inst C, Hangzhou 310020, Peoples R China
[3] Univ Witwatersrand, Sch Publ Hlth, Occupat Hlth Div, Parktown Educ Campus, ZA-2193 Johannesburg, South Africa
[4] Hangzhou Polytech, Inst Urban Construct, Hangzhou 311402, Peoples R China
[5] Sichuan Univ, Coll Architecture & Environm, Chengdu 610065, Peoples R China
基金
中国国家自然科学基金;
关键词
Indoor; Polybrominated diphenyl ethers (PBDEs); Settled dust; Exposure; Health risk; Urban China; BROMINATED FLAME-RETARDANTS; PERSISTENT ORGANIC POLLUTANTS; HAZARDOUS AIR-POLLUTANTS; IN-HOUSE DUST; HEALTH-RISK; POLYCHLORINATED-BIPHENYLS; INHALATION EXPOSURE; PHTHALATE EXPOSURE; PARTICLE-SIZE; PBDES;
D O I
10.1016/j.scitotenv.2020.136808
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this study, measurements of seven typical polybrominated diphenyl ethers (PBDEs) in indoor settled dust were summarized in selected urban regions of China. BDE-209 was the most dominant congener in settled dust (1.4-101 mu g/g), with a mean contribution of 95%. Indoor exposures to PBDEs were estimated via inhalation, dust ingestion, and dermal absorption. The average daily intake of Sigma PBDE was 4.9 to 19.1 ng/day/kg for all the population groups, with >80% of the total exposures from dust ingestion. Exposures in commuting environments (contributing 60%-80% of the total exposures) were higher than those in other microenvironments.The means of hazard indexes ranged from 1.66 x 10(-3) to 526 x 10(-3), which were mainly as a result of exposure to BDE-209, BDE-47, and BDE-99.The average lifetime cancer risks were from 0.03 x 10(-9) to 2.37 x 10(-9), which indicated the acceptable health risks resulting from indoor PBDE exposure for the Chinese population.The present study could provide valuable information that could be helpful for decision-makers, analysts and researchers to develop, implement and evaluate the effectiveness of interventions for the reduction of exposures to semi-volatile organic compounds (SVOCs) for large population groups in China. (C) 2020 Published by Elsevier B.V.
引用
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页数:10
相关论文
共 85 条
  • [1] [Anonymous], 2017, STOCKH CONV
  • [2] [Anonymous], EPA630R03003F RISK A
  • [3] [Anonymous], 2009, STOCKH CONV
  • [4] Concentrations and Emissions of Polybrominated Diphenyl Ethers from US Houses and Garages
    Batterman, Stuart A.
    Chernyak, Sergei
    Jia, Chunrong
    Godwin, Christopher
    Charles, Simone
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (08) : 2693 - 2700
  • [5] Children's Phthalate Intakes and Resultant Cumulative Exposures Estimated from Urine Compared with Estimates from Dust Ingestion, Inhalation and Dermal Absorption in Their Homes and Daycare Centers
    Beko, Gabriel
    Weschler, Charles J.
    Langer, Sarka
    Callesen, Michael
    Toftum, Jorn
    Clausen, Geo
    [J]. PLOS ONE, 2013, 8 (04):
  • [6] Human exposure to indoor air pollutants in sleep microenvironments: A literature review
    Boor, Brandon E.
    Spilak, Michal P.
    Laverge, Jelle
    Novoselac, Atila
    Xu, Ying
    [J]. BUILDING AND ENVIRONMENT, 2017, 125 : 528 - 555
  • [7] Polybrominated diphenyl ethers and novel brominated flame retardants in indoor dust of different microenvironments in Beijing, China
    Bu, Qingwei
    Wu, Dongkui
    Xia, Jing
    Wu, Min
    Liu, Xiaotu
    Cao, Zhiguo
    Yu, Gang
    [J]. ENVIRONMENT INTERNATIONAL, 2019, 122 : 159 - 167
  • [8] Exposure to commonly-used phthalates and the associated health risks in indoor environment of urban China
    Bu, Zhongming
    Mmereki, Daniel
    Wang, Jiahui
    Dong, Cong
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2019, 658 : 843 - 853
  • [9] Application of health information to hazardous air pollutants modeled in EPA's Cumulative Exposure Project
    Caldwell, JC
    Woodruff, TJ
    Morello-Frosch, R
    Axelrad, DA
    [J]. TOXICOLOGY AND INDUSTRIAL HEALTH, 1998, 14 (03) : 429 - 454
  • [10] Indoor particle age, a new concept for improving the accuracy of estimating indoor airborne SVOC concentrations, and applications
    Cao, Jianping
    Mo, Jinhan
    Sun, Zhiwei
    Zhang, Yinping
    [J]. BUILDING AND ENVIRONMENT, 2018, 136 : 88 - 97