Fabrication of novel hybrid Z-Scheme WO3@g-C3N4@MWCNT nanostructure for photocatalytic degradation of tetracycline and the evaluation of antimicrobial activity

被引:69
作者
Manikandan, V. S. [1 ]
Harish, S. [1 ]
Archana, J. [1 ]
Navaneethan, M. [1 ,2 ]
机构
[1] SRM Inst Sci & Technol, Dept Phys & Nanotechnol, Funct Mat & Energy Devices Lab, Kattankulathur Campus, Kattankulathur, Tamil Nadu, India
[2] SRM Inst Sci & Technol, Nanotechnol Res Ctr, Kattankulathur Campus, Kattankulathur, Tamil Nadu, India
关键词
Composites; WO3@g-C3N4; MWCNT; Hybrids; Degradation; WALLED CARBON NANOTUBES; G-C3N4; NANOSHEETS; GRAPHENE OXIDE; EFFICIENT; NANOCOMPOSITE; COMPOSITES; ANTIBACTERIAL; REMOVAL; PHOTODEGRADATION; NANOPARTICLES;
D O I
10.1016/j.chemosphere.2021.132050
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Exploring highly efficient visible-light-driven photocatalyst for the elimination organic pollutants is a great concern for constructing sustainable green energy systems. In the current work, a novel hybrid ternary WO3@gC3N4@MWCNT nanocomposites have been fabricated for visible-light-driven photocatalyst by self-assembly method. The as-prepared photocatalyst was examined by XRD, Raman, FESEM, HRTEM, XPS EDS, EIS, UV-visible DRS, and PL analysis. The experimental results revealed that the photocatalytic activity of WO3@gC3N4@MWCNT nanocomposites on the degradation of Tetracycline (TC) is 79.54% at 120 min, which is higher than the binary WO3@g-C3N4 composite and pristine WO3. The improved degradation performance towards TC is recognized for its higher surface area, intense light absorption towards the visible region, and enhanced charge separation efficiency. Consequently, the fabricated catalyst endows a promising application for antibiotic degradation.
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页数:10
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