Long-range transport and regional sources of PM2.5 in Beijing based on long-term observations from 2005 to 2010

被引:182
作者
Wang, Lili [1 ]
Liu, Zirui [1 ]
Sun, Yang [1 ]
Ji, Dongsheng [1 ]
Wang, Yuesi [1 ]
机构
[1] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China
基金
中国国家自然科学基金;
关键词
PM2.5; Long-range transport; Trajectory sector analysis; Potential source contribution function (PSCF); Beijing; PARTICULATE AIR-POLLUTION; ATMOSPHERIC AEROSOL; HAZE EPISODE; POLLUTANTS; SUMMER; PM10; QUALITY; TRENDS; CHINA; VISIBILITY;
D O I
10.1016/j.atmosres.2014.12.003
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Haze pollution in Beijing is rather deteriorated. Long-term measurement of PM2.5 from 2005 to 2010 at an urban site in Beijing showed very high concentration level with an annual average 74 +/- 55 mu g/m(3). The contribution of regional sources is one of the most important factors; thus, transport and regional sources of PM2.5 in Beijing are investigated using the trajectory cluster and receptor models (potential source contribution function and trajectory sector analysis). The results indicated that the highest concentrations of PM2.5 (76-120 mu g/m(3)) were associated with south, southeast, and short northwest trajectories, and moderate concentrations (46-67 mu g/m(3)) with long northwest and short north trajectories, and the lowest concentrations (20-33 mu g/m(3)) with long north trajectories. During the relatively polluted periods, the probable locations of regional emission sources were mainly in the south and the west of Beijing and varied according to different seasons. Between 2005 and 2010, the annual mean contribution of 35.5% (32.8 mu g/m(3)) for PM2.5 was attributed to long-distance transportation. The transported contribution percentages from 2005 to 2010 for PM2.5 showed an increasing tendency with a linear rate of 1.2/year. (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:37 / 48
页数:12
相关论文
共 56 条
[41]   Analysis of the dependence of column-integrated aerosol properties on long-range transport of air masses in Beijing [J].
Xia, X. ;
Chen, H. ;
Zhang, W. .
ATMOSPHERIC ENVIRONMENT, 2007, 41 (36) :7739-7750
[42]   The empirical relationship between the PM2.5 concentration and aerosol optical depth over the background of North China from 2009 to 2011 [J].
Xin, Jinyuan ;
Zhang, Qing ;
Wang, Lili ;
Gong, Chongshui ;
Wang, Yuesi ;
Liu, Zirui ;
Gao, Wenkang .
ATMOSPHERIC RESEARCH, 2014, 138 :179-188
[43]   Reductions of PM2.5 in Beijing-Tianjin-Hebei urban agglomerations during the 2008 Olympic Games [J].
Xin Jinyuan ;
Wang Yuesi ;
Wang Lili ;
Tang Guiqian ;
Sun Yang ;
Pan Yuepeng ;
Ji Dongsheng .
ADVANCES IN ATMOSPHERIC SCIENCES, 2012, 29 (06) :1330-1342
[44]   Variability and reduction of atmospheric pollutants in Beijing and its surrounding area during the Beijing 2008 Olympic Games [J].
Xin JinYuan ;
Wang YueSi ;
Tang GuiQian ;
Wang LiLi ;
Sun Yang ;
Wang YingHong ;
Hu Bo ;
Song Tao ;
Ji DongSheng ;
Wang WeiFeng ;
Li Liang ;
Liu GuangRen .
CHINESE SCIENCE BULLETIN, 2010, 55 (18) :1937-1944
[45]  
Xu XH, 2008, AEROSOL AIR QUAL RES, V8, P78
[46]   A comparative analysis of aerosol properties in dust and haze-fog days in a Chinese urban region [J].
Yu, Xingna ;
Zhu, Bin ;
Yin, Yan ;
Yang, Jun ;
Li, Yanwei ;
Bu, Xiaoli .
ATMOSPHERIC RESEARCH, 2011, 99 (02) :241-247
[47]   Ambient air quality trends and driving factor analysis in Beijing, 1983-2007 [J].
Zhang, Ju ;
Ouyang, Zhiyun ;
Miao, Hong ;
Wang, Xiaoke .
JOURNAL OF ENVIRONMENTAL SCIENCES, 2011, 23 (12) :2019-2028
[48]   A health-based assessment of particulate air pollution in urban areas of Beijing in 2000-2004 [J].
Zhang, Minsi ;
Song, Yu ;
Cai, Xuhui .
SCIENCE OF THE TOTAL ENVIRONMENT, 2007, 376 (1-3) :100-108
[49]   The challenge of improving visibility in Beijing [J].
Zhang, Q. H. ;
Zhang, J. P. ;
Xue, H. W. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (16) :7821-7827
[50]   Chemical characterization and source apportionment of PM2.5 in Beijing: seasonal perspective [J].
Zhang, R. ;
Jing, J. ;
Tao, J. ;
Hsu, S. -C. ;
Wang, G. ;
Cao, J. ;
Lee, C. S. L. ;
Zhu, L. ;
Chen, Z. ;
Zhao, Y. ;
Shen, Z. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2013, 13 (14) :7053-7074