Efficient Full-Color Boron Nitride Quantum Dots for Thermostable Flexible Displays

被引:49
|
作者
Ding, Yamei [1 ]
He, Ping [1 ]
Li, Shaohan [1 ]
Chang, Bo [1 ]
Zhang, Shengli [2 ]
Wang, Zhehan [1 ]
Chen, Jiayi [1 ,3 ]
Yu, Jin [1 ]
Wu, Sanxie [4 ]
Zeng, Haibo [2 ]
Tao, Li [1 ,3 ,5 ]
机构
[1] Southeast Univ, Sch Mat Sci & Engn, Jiangsu Key Lab Adv Metall Mat, Nanjing 211189, Peoples R China
[2] Nanjing Univ Sci & Technol, Minist Ind & Informat Technol, Key Lab Adv Display Mat & Devices, Coll Mat Sci & Engn, Nanjing 210094, Peoples R China
[3] Southeast Univ, Ctr 2D Mat, Nanjing 211189, Peoples R China
[4] Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210023, Peoples R China
[5] Southeast Univ, Ctr Flexible RF Technol, Nanjing 211189, Peoples R China
基金
中国国家自然科学基金;
关键词
hexagonal boron nitride; quantum dots; full-color emission; quantum yield; flexible displays; CARBON DOTS; PHOTOLUMINESCENCE; LUMINESCENCE; FABRICATION; NANOSHEETS; SURFACE; FACILE;
D O I
10.1021/acsnano.1c04321
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Hexagonal boron nitride quantum dot (BNQD) has aroused great interest in the optoelectronics field due to their metal-free nature with promising optical properties. However, it has been a great challenge to modulate its photoluminescence to the long-wavelength region so far. Herein, BNQDs with full-color emission (420-610 nm) have been implemented by doping diverse amino ligands in different solvents for the first attempt. This color variation from blue, green, yellow-green, yellow to red is ascribed to the surface states tunable via amination degree. Attractively, the quantum yield of our blue BNQDs has set a record at 32.27%, and rare yellow-green BNQDs have been demonstrated. Combining good thermal dissipation capability and high transparency, our fullcolor BNQD holds great potential for transparent flexible display and security labels at the elevated temperature.
引用
收藏
页码:14610 / 14617
页数:8
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