Vertical distributions of SO2 and NO2 in the lower atmosphere in Beijing urban areas, China

被引:82
作者
Meng, Z. Y. [1 ]
Ding, G. A. [1 ]
Xu, X. B. [1 ]
Xu, X. D. [1 ]
Yu, H. Q. [2 ]
Wang, S. F. [1 ]
机构
[1] China Meteorol Adm, Chinese Acad Meteorol Sci, Ctr Atmospher Watch & Serv, Key Lab Atmospher Chem, Beijing 100081, Peoples R China
[2] China Meteorol Adm, Natl Meteorol Ctr, Beijing 100081, Peoples R China
关键词
sulfur dioxide; nitrogen dioxide; vertical distribution; passive sampler; meteorological conditions;
D O I
10.1016/j.scitotenv.2007.10.012
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Measurements of SO2 and NO2 were conducted from January to March 2001 and August 2003 at a 325 in meteorological tower in Beijing. The concentrations of SO2 and NO2 observed by passive samplers at ten heights showed complex vertical distributions in winter and summer. The vertical profiles of pollutants were influenced by source emissions, meteorological conditions, urban canopy and other factors. The comparison analysis of winter and summer pollutant concentrations suggests that the decrease in SO2 concentration was significant in summer, and the reduction of NO2 was relatively not distinctive. Domestic heating and industrial sources were major sources of SO2 in urban areas of Beijing. Differing from SO2 urban NO2 was closely related to traffic emission. Meteorological evidence suggests that strong temperature inversions influence vertical distribution of air pollutants over urban Beijing. The high levels of SO2 and NO2 concentrations were due to the accumulation of pollutants resulting from the stable atmosphere prevalent during the measurement period. The vertical distributions of air pollutants were controlled and affected by atmospheric dynamical characteristics. (c) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:456 / 465
页数:10
相关论文
共 34 条
[1]   Indoor and outdoor air pollution in Tokyo and Beijing supercities [J].
Ando, M ;
Katagiri, K ;
Tamura, K ;
Yamamoto, S ;
Matsumoto, M ;
Li, YF ;
Cao, SR ;
Ji, RD ;
Liang, CK .
ATMOSPHERIC ENVIRONMENT, 1996, 30 (05) :695-702
[2]   SPATIAL AND TEMPORAL VARIATION OF RURAL NITROGEN-DIOXIDE CONCENTRATIONS ACROSS THE UNITED-KINGDOM [J].
ATKINS, DHF ;
LEE, DS .
ATMOSPHERIC ENVIRONMENT, 1995, 29 (02) :223-239
[3]   Validation of passive diffusion samplers for SO2 and NO2 [J].
Ayers, GP ;
Keywood, MD ;
Gillett, R ;
Manins, PC ;
Malfroy, H ;
Bardsley, T .
ATMOSPHERIC ENVIRONMENT, 1998, 32 (20) :3587-3592
[4]   Measurements of sulfur dioxide, ozone and ammonia concentrations in Asia, Africa, and South America using passive samplers [J].
Carmichael, GR ;
Ferm, M ;
Thongboonchoo, N ;
Woo, JH ;
Chan, LY ;
Murano, K ;
Viet, PH ;
Mossberg, C ;
Bala, R ;
Boonjawat, J ;
Upatum, P ;
Mohan, M ;
Adhikary, SP ;
Shrestha, AB ;
Pienaar, JJ ;
Brunke, EB ;
Chen, T ;
Jie, T ;
Guoan, D ;
Peng, LC ;
Dhiharto, S ;
Harjanto, H ;
Jose, AM ;
Kimani, W ;
Kirouane, A ;
Lacaux, JP ;
Richard, S ;
Barturen, O ;
Cerda, JC ;
Athayde, A ;
Tavares, T ;
Cotrina, JS ;
Bilici, E .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (9-10) :1293-1308
[5]   Characteristics of vertical profiles and sources of PM2.5, PM10 and carbonaceous species in Beijing [J].
Chan, CY ;
Xu, XD ;
Li, YS ;
Wong, KH ;
Ding, GA ;
Chan, LY ;
Cheng, XH .
ATMOSPHERIC ENVIRONMENT, 2005, 39 (28) :5113-5124
[6]   ANALYSIS AND INTERPRETATION OF AIR-QUALITY DATA FROM AN URBAN ROADSIDE LOCATION IN CENTRAL LONDON OVER THE PERIOD FROM JULY 1991 TO JULY 1992 [J].
DERWENT, RG ;
MIDDLETON, DR ;
FIELD, RA ;
GOLDSTONE, ME ;
LESTER, JN ;
PERRY, R .
ATMOSPHERIC ENVIRONMENT, 1995, 29 (08) :923-946
[7]  
DING G, 2002, J APPL METEOROLOGICA, V13, P82
[8]   Vertical structures of PM10 and PM 2.5 and their dynamical character in low atmosphere in Beijing urban areas [J].
Ding, GA ;
Chan, CY ;
Gao, ZQ ;
Yao, WQ ;
Li, YS ;
Cheng, XH ;
Meng, ZY ;
Yu, HQ ;
Wong, K ;
Wang, SF ;
Miao, QJ .
SCIENCE IN CHINA SERIES D-EARTH SCIENCES, 2005, 48 :38-54
[9]   Simulation of meteorological fields within and above urban and rural canopies with a mesoscale model (MM5) [J].
Dupont, S ;
Otte, TL ;
Ching, JKS .
BOUNDARY-LAYER METEOROLOGY, 2004, 113 (01) :111-158
[10]   Cost-efficient techniques for urban- and background measurements of SO2 and NO2 [J].
Ferm, M ;
Svanberg, PA .
ATMOSPHERIC ENVIRONMENT, 1998, 32 (08) :1377-1381