Adsorption-photodegradation synergetic removal of methylene blue from aqueous solution by NiO/graphene oxide nanocomposite

被引:63
作者
Rong, Xinshan [1 ]
Qiu, Fengxian [2 ]
Zhang, Chen [2 ]
Fu, Liang [2 ]
Wang, Yuanyuan [2 ]
Yang, Dongya [2 ]
机构
[1] Jiangsu Univ, Sch Environm & Safety Engn, Zhenjiang 212013, Peoples R China
[2] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China
关键词
Adsorption; Photodegradation; Nanocomposite; Removal efficiency; LITHIUM-ION BATTERIES; ENHANCED PHOTOCATALYTIC PERFORMANCE; MALACHITE GREEN; GRAPHENE OXIDE; NIO; DEGRADATION; DYE; NANOPARTICLES; HYBRID; FIBERS;
D O I
10.1016/j.powtec.2015.01.079
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Nickel oxide/graphene oxide (NiO/GO) nanocomposite was prepared by a hydrothermal method combining a subsequent calcination process. X-ray diffraction (XRD), Raman spectrometer (Raman), high resolution transmission electron microscopy (HRTEM), selected area electron diffraction (SAED) and X-ray photoelectron spectroscopy (XPS) methods were used for the characterization of nanocomposite. Removal of aromatic heterocyclic dye methylene blue (MB) from aqueous solution using adsorption and photodegradation activity of NiO/GO nanocomposite was investigated. The effects of NiO/GO nanocomposite dose, pH, and contact time on the removal efficiency of MB were also investigated. Compared with that in the dark, NiO/GO nanocomposite shows a faster and higher removal efficiency by the photodegradation and adsorption under visible light irradiation. A remarkable removal efficiency of MB achieved 97.54% by NiO/GO nanocomposite after 2 h. It could be concluded that synergy of photodegradation and adsorption has a significant progress for removal of MB under visible light compared with that of only adsorption without light. (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:322 / 328
页数:7
相关论文
共 28 条
  • [1] Honeycomb Carbon: A Review of Graphene
    Allen, Matthew J.
    Tung, Vincent C.
    Kaner, Richard B.
    [J]. CHEMICAL REVIEWS, 2010, 110 (01) : 132 - 145
  • [2] Synthesis of reduced graphene oxide/α-Bi2Mo3O12 @ β-Bi2O3 heterojunctions by organic electrolytes assisted UV-excited method
    Cao, Shiyi
    Chen, Chuansheng
    Liu, Tiangui
    Tsang, Yuenhong
    Zhang, Xuming
    Yu, Weiwei
    Chen, Weiwei
    [J]. CHEMICAL ENGINEERING JOURNAL, 2014, 257 : 309 - 316
  • [3] Influence of pH on the specific surface area of polyaniline matrices
    Chowdhury, Al-Nakib
    Saleh, Farhana Sultana
    Rahman, Mohammad Rezaur
    Rahim, Abdur
    [J]. JOURNAL OF APPLIED POLYMER SCIENCE, 2008, 109 (03) : 1764 - 1771
  • [4] Single-crystalline porous NiO nanosheets prepared from β-Ni(OH)2 nanosheets: Magnetic property and photocatalytic activity
    Dong, Qiang
    Yin, Shu
    Guo, Chongshen
    Wu, Xiaoyong
    Kumada, Nobuhiro
    Takei, Takahiro
    Miura, Akira
    Yonesaki, Yoshinori
    Sato, Tsugio
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2014, 147 : 741 - 747
  • [5] Catalytic Degradation of an Organic Dye through Electroreduction of Dioxygen in Aqueous Solution
    Farhana, Tamanna Ishrat
    Mollah, M. Yousuf Ali
    Susan, Md Abu Bin Hasan
    Islam, Md. Mominul
    [J]. ELECTROCHIMICA ACTA, 2014, 139 : 244 - 249
  • [6] Facile preparation of graphene supported Co3O4 and NiO for reducing fire hazards of polyamide 6 composites
    Hong, Ningning
    Song, Lei
    Hull, T. Richard
    Stec, Anna A.
    Wang, Bibo
    Pan, Ying
    Hu, Yuan
    [J]. MATERIALS CHEMISTRY AND PHYSICS, 2013, 142 (2-3) : 531 - 538
  • [7] Photocatalytic degradation pathway of methylene blue in water
    Houas, A
    Lachheb, H
    Ksibi, M
    Elaloui, E
    Guillard, C
    Herrmann, JM
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 2001, 31 (02) : 145 - 157
  • [8] Rapid microwave-assisted synthesis of graphene nanosheets-zinc sulfide nanocomposites: Optical and photocatalytic properties
    Hu, Huating
    Wang, Xianbao
    Liu, Fangming
    Wang, Jingchao
    Xu, Chunhui
    [J]. SYNTHETIC METALS, 2011, 161 (5-6) : 404 - 410
  • [9] Utilization of bivalve shell-treated Zea mays L. (maize) husk leaf as a low-cost biosorbent for enhanced adsorption of malachite green
    Jalil, A. A.
    Triwahyono, S.
    Yaakob, M. R.
    Azmi, Z. Z. A.
    Sapawe, N.
    Kamarudin, N. H. N.
    Setiabudi, H. D.
    Jaafar, N. F.
    Sidik, S. M.
    Adam, S. H.
    Hameed, B. H.
    [J]. BIORESOURCE TECHNOLOGY, 2012, 120 : 218 - 224
  • [10] A facile hydrothermal synthesis of graphene porous NiO nanocomposite and its application in electrochemical capacitors
    Jiang, Yong
    Chen, Dandan
    Song, Jinsong
    Jiao, Zheng
    Ma, Qiliang
    Zhang, Haijiao
    Cheng, Lingli
    Zhao, Bing
    Chu, Yuliang
    [J]. ELECTROCHIMICA ACTA, 2013, 91 : 173 - 178