An efficient flexible electrochemical glucose sensor based on carbon nanotubes/carbonized silk fabrics decorated with Pt microspheres

被引:117
作者
Chen, Chao [1 ]
Ran, Rui [1 ]
Yang, Zhiyu [1 ]
Lv, Ruitao [1 ]
Shen, Wanci [1 ]
Kang, Feiyu [1 ,3 ]
Huang, Zheng-Hong [1 ,2 ]
机构
[1] Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
[2] Tsinghua Univ, Sch Mat Sci & Engn, Key Lab Adv Mat MOE, Beijing 100084, Peoples R China
[3] Tsinghua Univ, Grad Sch Shenzhen, Shenzhen 518055, Peoples R China
基金
中国国家自然科学基金;
关键词
Flexible sensor; Carbonized silk fabric; Pt microspheres; Glucose; DIRECT ELECTRON-TRANSFER; GRAPHENE; OXIDASE; ADSORPTION; NANOTUBES; SURFACE; IMMOBILIZATION; NANOPARTICLES; PERFORMANCE; PROTEIN;
D O I
10.1016/j.snb.2017.10.067
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Advanced flexible electronics have been attracting increasing attention nowadays. Herein, we fabricated an efficient flexible glucose sensor based on multi-walled carbon nanotubes coated carbonized silk fabric (MWCNTs/CSF) by Pt microsphere decoration. The MWCNTs/CSF was obtained by carbonization at 950 degrees C under an inert atmosphere, which showed good conductivity, flexibility and stability. After a decoration of Pt microspheres by electrodeposition, the resultant material showed a good sensitivity towards H2O2. Following with immobilizing with glucose oxidase (GOx), the resultant sensor showed a sensitivity of 288.86 mu A mM(-1) cm(-2) with a good linear range from 0 to 5 mM. This method is considered to be an efficient way to fabricate flexible electrodes and wearable electronic devices. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:63 / 70
页数:8
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