Liquid Organic Frameworks: The Single-Network "Plumber's Nightmare" Bicontinuous Cubic Liquid Crystal

被引：33

作者：

Poppe, Silvio ^{[3
]}

Cheng, Xiaohong ^{[3
,4
]}

Chen, Changlong ^{[1
]}

Zeng, Xiangbing ^{[2
]}

Zhang, Rui-bin ^{[2
]}

Liu, Feng ^{[1
]}

Ungar, Goran ^{[1
,2
]}

Tschierske, Carsten ^{[3
]}

机构：

[1] Xi An Jiao Tong Univ, Shaanxi Int Res Ctr Soft Matter, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China

[2] Univ Sheffield, Dept Mat Sci & Engn, Sheffield S1 3JD, S Yorkshire, England

[3] Martin Luther Univ Halle Wittenberg, Inst Chem, D-06120 Halle, Germany

[4] Yunnan Univ, Key Lab Med Chem Nat Resources, Chem Dept, Kunming 650091, Yunnan, Peoples R China

来源：

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY | 2020年 / 142卷 / 07期

基金：

中国国家自然科学基金; 英国工程与自然科学研究理事会;

关键词：

PHASE;

D O I：

10.1021/jacs.9b11073

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Novel bolapolyphiles, built of a p-terphenyl or bistolane core with polar glycerol end-groups and two laterally attached n-alkyl or semiperfluoroalkyl chains, form the first "single plumber's nightmare network", the simplest soft-matter cubic phase (Pm (3) over barm). Its cage-like grid comprises bundles of aromatic rods lying along the cubic unit cell edges, connected by six-way hydrogen-bonded junctions. Side-chains fill the remaining volume of this unique noninterpenetrating liquid-crystalline organic framework.

引用

页码：3296 / 3300

页数：5

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