Fabrication, optical and scintillation properties of transparent YAG:Ce ceramics

被引:47
作者
Osipov, V. V. [1 ]
Ishchenko, A. V. [2 ]
Shitov, V. A. [1 ]
Maksimov, R. N. [1 ,2 ]
Lukyashin, K. E. [1 ]
Platonov, V. V. [1 ]
Orlov, A. N. [1 ]
Osipov, S. N. [2 ]
Yagodin, V. V. [2 ]
Viktorov, L. V. [2 ]
Shulgin, B. V. [2 ]
机构
[1] RAS, Inst Electrophys UrB, Ekaterinburg 620016, Russia
[2] Ural Fed Univ, Ekaterinburg 620002, Russia
关键词
Transparent ceramics; Scintillator; Laser ablation; Nanopowder; Yttrium aluminium garnet; Cerium; SINGLE-CRYSTAL; LUMINESCENCE; NANOPOWDERS; DETECTORS; PHOSPHOR;
D O I
10.1016/j.optmat.2016.05.016
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Highly transparent YAG:Ce ceramics (transmission of 72-82% for 2-mm-thick samples in 550-900 nm wavelength range) were fabricated by solid-state reactive sintering using a mixture of Ce2xY2-2xO3 (x = 0.001, 0.01, 0.03, and 0.05) and Al2O3 nanopowders synthesized by laser ablation with an additional round of pre-calcining before compaction. The synthesized YAG:Ce ceramic materials showed intense luminescence with a maximum at 525-545 nm. The measured absolute light yields of the synthesized YAG:Ce ceramics were 18-21 photon/MeV for 1-5 at.% Ce and 5 photon/MeV for 0.1 at.% Ce. The energy resolutions of the fabricated thin ceramic samples (2 mm) under 662 keV gamma ray were measured to be 10-15%. The decay curves of scintillations consisted of two components with the decay times depending on the Ce3+ concentration. The sample doped with 5 at.% of Ce exhibited the main fast component with 26 ns decay time. The measured data was compared to that of YAG:Ce and well-known CsI:T1 single crystal scintillators. The influence of dopant concentration on the optical, luminescence and scintillation properties was discussed. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:98 / 102
页数:5
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