Compositional dependence of the magnetic state of Co3-xZnxTeO6 solid solutions

被引：3
作者：
Sarkar, T. [1 ]
Ivanov, S. A. [1 ,2 ]
Weil, M. [3 ]
Clulow, R. [4 ]
Lewin, E. [4 ]
Mathieu, R. [1 ]
机构：
[1] Uppsala Univ, Dept Mat Sci & Engn, Box 35, SE-75103 Uppsala, Sweden
[2] Moscow MV Lomonosov State Univ, Dept Chem, Leninskie Gory 1-3, Moscow 119991, Russia
[3] Vienna Univ Technol, Inst Chem Technol & Analyt, A-1060 Vienna, Austria
[4] Uppsala Univ, Dept Chem, Angstrom Lab, S-75121 Uppsala, Sweden
来源：
JOURNAL OF ALLOYS AND COMPOUNDS | 2021年 / 884卷
基金：
瑞典研究理事会;
关键词：
Magnetic oxides; Magnetic dilution; Structure-property correlations; Strongly correlated systems; CRYSTAL; SPIN;
D O I：
10.1016/j.jallcom.2021.161111
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The magnetic properties of phase-pure solid solutions of Co3-xZnxTeO6 are investigated using magnetometry (single crystals) and neutron diffraction (polycrystalline powders), and compared to results of detailed crystallographic studies. There are five unique Co sites in Co3TeO6, including a tetrahedrally coordinated Co-2 site which Zn preferentially occupies. The magnetic interaction is found to monotonically decrease as the Co-2-O bond length decreases with increasing Zn content. The results suggest a modification of the magnetic structure in the samples containing Zn. (C) 2021 The Author(s). Published by Elsevier B.V.
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页数：6
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