Breakthrough of Organic Electroluminescence Efficiency of Photoluminescence in Frequency Domain

被引:1
作者
Huang, Jin-Zhao [1 ]
Li, Shi-Shuai [1 ]
Feng, Xiu-Peng [1 ]
Wang, Pei-Ji [1 ]
Zhang, Zhong [1 ]
机构
[1] Univ Jinan, Sch Sci, Jinan 250022, Shandong, Peoples R China
关键词
Frequency domain; 25 % Limitation; Triplet; Singlet; TRIPLET EXCITON FORMATION; SINGLET;
D O I
暂无
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this paper, a new way is proposed to confirm that the organic electroluminescence efficiency can exceed the 25 % limitation of that of photoluminescence in frequency domain. In present experiment, the spectra shows two characteristic emission bands and the high and low energy emission bands are due to singlet and triplet excited states. The triplet emission has longer lifetime than that of singlet emission and the emission intensity of short lifetime changes (increase and decrease)more dramatic than that of long lifetime with the changing frequency. So, it may be concluded that the 25 % limitation is not perfect and can be exceeded in the frequency domain at a given frequency.
引用
收藏
页码:4688 / 4692
页数:5
相关论文
共 15 条
  • [1] Chain-length dependence of singlet and triplet exciton formation rates in organic light-emitting diodes
    Beljonne, D
    Ye, AJ
    Shuai, Z
    Brédas, JL
    [J]. ADVANCED FUNCTIONAL MATERIALS, 2004, 14 (07) : 684 - 692
  • [2] Improved quantum efficiency for electroluminescence in semiconducting polymers
    Cao, Y
    Parker, ID
    Yu, G
    Zhang, C
    Heeger, AJ
    [J]. NATURE, 1999, 397 (6718) : 414 - 417
  • [3] Triplet formation and decay in conjugated polymer devices
    Dhoot, AS
    Ginger, DS
    Beljonne, D
    Shuai, Z
    Greenham, NC
    [J]. CHEMICAL PHYSICS LETTERS, 2002, 360 (3-4) : 195 - 201
  • [4] Quantum molecular dynamics study of polaron recombination in conjugated polymers
    Kobrak, MN
    Bittner, ER
    [J]. PHYSICAL REVIEW B, 2000, 62 (17) : 11473 - 11486
  • [5] Triplet-to-singlet exciton formation in poly(p-phenylene-vinylene) light-emitting diodes -: art. no. 036601
    Lin, LC
    Meng, HF
    Shy, JT
    Horng, SF
    Yu, LS
    Chen, CH
    Liaw, HH
    Huang, CC
    Peng, KY
    Chen, SA
    [J]. PHYSICAL REVIEW LETTERS, 2003, 90 (03) : 4
  • [6] Lu J, 2007, SPECTROSC SPECT ANAL, V27, P420
  • [7] Singlet and triplet exciton formation rates in conjugated polymer light-emitting diodes
    Shuai, Z
    Beljonne, D
    Silbey, RJ
    Brédas, JL
    [J]. PHYSICAL REVIEW LETTERS, 2000, 84 (01) : 131 - 134
  • [8] Activator recycling in low voltage cathodoluminescent phosphors
    Stoffers, C
    Yang, S
    Zhang, F
    Jacobsen, SM
    Wagner, BK
    Summers, CJ
    [J]. APPLIED PHYSICS LETTERS, 1997, 71 (13) : 1759 - 1761
  • [9] Electron correlation effects in electron-hole recombination in organic light-emitting diodes
    Tandon, K
    Ramasesha, S
    Mazumdar, S
    [J]. PHYSICAL REVIEW B, 2003, 67 (04)
  • [10] Spin-dependent exciton formation in π-conjugated compounds
    Wilson, JS
    Dhoot, AS
    Seeley, AJAB
    Khan, MS
    Köhler, A
    Friend, RH
    [J]. NATURE, 2001, 413 (6858) : 828 - 831