Cross section measurements of deuteron induced nuclear reactions on natural tungsten up to 34 MeV

被引：23
作者：
Duchemin, C. [1 ]
Guertin, A. [1 ]
Haddad, F. [1 ,2 ]
Michel, N. [1 ,2 ]
Metivier, V. [1 ]
机构：
[1] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS,IN2P3, Nantes, France
[2] GIP Arronax, F-44817 St Herblain, France
来源：
APPLIED RADIATION AND ISOTOPES | 2015年 / 97卷
关键词：
Tungsten target; Deuteron beam; Stacked-foil technique; Excitation function; TALYS; 1.6; EXCITATION-FUNCTIONS; ARRONAX; ACTIVATION;
D O I：
10.1016/j.apradiso.2014.12.011
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Re-196g is a beta-/gamma emitter of great interest for nuclear medicine. It has shown successful results on bone metastases palliation and has similar chemical properties as Tc-99m, the most commonly used imaging agent. Re-196g is routinely produced using rhenium target in nuclear reactor. Higher specific activity could be obtained using accelerators. In this paper, production cross section values are presented for the W-nat(d, x)Re-196g reaction up to 34 MeV, using the stacked-foils method and gamma spectrometry. From this data set, the thick target production yield of Re-196g is determined and compared with the validated values of the IAEA and also with the proton route. The production cross sections of the W-nat(d, x)Re-183,Re-182g,Re-184m,Re-184g,Re-181 and W-nat(d, x)W-187 reactions have also been determined. A good agreement is found with the literature. Our data are compared with the version 1.6 (December 2013) of the TALYS code which shows discrepancies both on the shape and on the amplitude for these deuteron induced reactions. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码：52 / 58
页数：7
相关论文
共 22 条
[1]   EXCITATION FUNCTIONS FOR THE W-184(D,P)W-185, W-186(D,P)W-187 AND W-184(D,2N) RE-184 REACTIONS - AND HALF LIVES OF W-185 AND W-187 [J].
ANDELIN, RL .
JOURNAL OF INORGANIC & NUCLEAR CHEMISTRY, 1964, 26 (06) :1117-1120
[2]   INTERNAL IRRADIATION SYSTEM FOR EXCITATION-FUNCTION MEASUREMENT VIA THE STACKED-FOIL TECHNIQUE [J].
BLESSING, G ;
BRAUTIGAM, W ;
BOGE, HG ;
GAD, N ;
SCHOLTEN, B ;
QAIM, SM .
APPLIED RADIATION AND ISOTOPES, 1995, 46 (09) :955-960
[3]   Production study of high specific activity NCA Re-186g by proton and deuteron cyclotron irradiation [J].
Bonardi, M. L. ;
Groppi, F. ;
Manenti, S. ;
Persico, E. ;
Gini, L. .
APPLIED RADIATION AND ISOTOPES, 2010, 68 (09) :1595-1601
[4]   232Th(d,4n) 230Pa cross-section measurements at ARRONAX facility for the production of 230U [J].
Duchemin, C. ;
Guertin, A. ;
Haddad, F. ;
Michel, N. ;
Metivier, V. .
NUCLEAR MEDICINE AND BIOLOGY, 2014, 41 :E19-E22
[5]   Experience with aluminum perrhenate targets for reactor production of high specific activity Re-186 [J].
Ehrhardt, GJ ;
Blumer, ME ;
Su, FM ;
Vanderheyden, JL ;
Fritzberg, AR .
APPLIED RADIATION AND ISOTOPES, 1997, 48 (01) :1-4
[6]   Reactor-produced radionuclides at the University of Missouri Research Reactor [J].
Ehrhardt, GJ ;
Ketring, AR ;
Ayers, LM .
APPLIED RADIATION AND ISOTOPES, 1998, 49 (04) :295-297
[7]  
Ekstrom L.F., 2004, INFORM EXTRACTED TAB
[8]  
Gobin R., 2009, P ICIS09 GATL TENN U
[9]   Measurements of 186Re production cross section induced by deuterons on natW target at ARRONAX facility [J].
Guertin, Arnaud ;
Duchemin, Charlotte ;
Haddad, Ferid ;
Michel, Nathalie ;
Metivier, Vincent .
NUCLEAR MEDICINE AND BIOLOGY, 2014, 41 :E16-E18
[10]   ARRONAX, a high-energy and high-intensity cyclotron for nuclear medicine [J].
Haddad, Ferid ;
Ferrer, Ludovic ;
Guertin, Arnaud ;
Carlier, Thomas ;
Michel, Nathalie ;
Barbet, Jacques ;
Chatal, Jean-Francois .
EUROPEAN JOURNAL OF NUCLEAR MEDICINE AND MOLECULAR IMAGING, 2008, 35 (07) :1377-1387
123