Biodegradable Natural Pectin-Based Polysaccharide-Gated Low-Voltage Flexible Oxide Thin-Film Transistors for Logic Applications

被引:2
作者
Liu, Yanghui [1 ]
Li, Fangzhou [1 ]
Guo, Jianmiao [1 ]
Liang, Linzi [1 ]
Liu, Kekang [1 ]
Liu, Ning [2 ]
机构
[1] Sun Yat Sen Univ, Sch Mat, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Peoples R China
[2] Nanchang Inst Technol, Sch Sci, Nanchang 330029, Peoples R China
关键词
biodegradable; electric double layer; flexible electronics; logic gates; oxide thinffilm transistors;
D O I
10.1021/acsaelm.2c00687
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Electronic waste is one of the fastest growing kinds of waste in the world, and to reduce which, the biodegradable electronics are regarded as an important eco-friendly alternative to the environmentally hazardous ones. Here, biodegradable indium-tin-oxide (ITO) thin-film transistors (TFTs) are fabricated on flexible PET substrates with pectin-based polysaccharide films taken as gate dielectrics. For the basic performance, such biodegradable TFTs have not only exhibited excellent characteristics such as a low operating voltage of 1.0 V, a high current ON/OFF ratio (> 10(7)), a low subthreshold swing of 80 mV/dec, and a carrier mobility of 14.5 cm(2)V(-1) s(-1), but have also realized several important logic operations, such as NOT, AND, NAND, and so on. Additionally, for the eco-friendly purpose, the TFT arrays can be completely dissolved in water within 20 min. Based on the results achieved, the pectin-based biodegradable oxide transistors prepared here are expected to provide a possible choice for the fabrication of biodegradable electronics by using natural biomaterials.
引用
收藏
页码:4061 / 4067
页数:7
相关论文
共 37 条
[1]   Materials and processing approaches for foundry-compatible transient electronics [J].
Chang, Jan-Kai ;
Fang, Hui ;
Bower, Christopher A. ;
Song, Enming ;
Yu, Xinge ;
Rogers, John A. .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2017, 114 (28) :E5522-E5529
[2]   Modeling Novel Double-in-Plane Gate Electric-Double-Layer Thin-Film and Nanoscale Transistors [J].
Dai, Mingzhi ;
Wan, Qing .
NANO LETTERS, 2011, 11 (09) :3987-3990
[3]   Determination of pectin degree of esterification by diffuse reflectance Fourier transform infrared spectroscopy [J].
Gnanasambandam, R ;
Proctor, A .
FOOD CHEMISTRY, 2000, 68 (03) :327-332
[4]   Linear Classification Function Emulated by Pectin-Based Polysaccharide-Gated Multiterminal Neuron Transistors [J].
Guo, Jianmiao ;
Liu, Yanghui ;
Zhou, Feichi ;
Li, Fangzhou ;
Li, Yingtao ;
Huang, Feng .
ADVANCED FUNCTIONAL MATERIALS, 2021, 31 (33)
[5]   Bienenstock-Cooper-Munro Learning Rule Realized in Polysaccharide-Gated Synaptic Transistors with Tunable Threshold [J].
Guo, Jianmiao ;
Liu, Yanghui ;
Li, Yingtao ;
Li, Fangzhou ;
Huang, Feng .
ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (44) :50061-50067
[6]   Logic gates and computation from assembled nanowire building blocks [J].
Huang, Y ;
Duan, XF ;
Cui, Y ;
Lauhon, LJ ;
Kim, KH ;
Lieber, CM .
SCIENCE, 2001, 294 (5545) :1313-1317
[7]   All-Solid-State Organic Schmitt Trigger Implemented by Twin Two-in-One Ferroelectric Memory Transistors [J].
Hwang, Sunbin ;
Jang, Sukjae ;
Bae, Sukang ;
Lee, Seoung-Ki ;
Lee, Sang Hyun ;
Fabiano, Simone ;
Berggren, Magnus ;
Lee, Takhee ;
Kim, Tae-Wook .
ADVANCED ELECTRONIC MATERIALS, 2020, 6 (05)
[9]   Transparent Junctionless Electric-Double-Layer Transistors Gated by a Reinforced Chitosan-Based Biopolymer Electrolyte [J].
Jiang, Jie ;
Wan, Qing ;
Zhang, Qing .
IEEE TRANSACTIONS ON ELECTRON DEVICES, 2013, 60 (06) :1951-1957
[10]   Printable ion-gel-gated In2O3 synaptic transistor array for neuro-inspired memory [J].
Jin, Chenxing ;
Liu, Wanrong ;
Huang, Yulong ;
Xu, Yunchao ;
Nie, Yiling ;
Zhang, Gengming ;
He, Pei ;
Sun, Jia ;
Yang, Junliang .
APPLIED PHYSICS LETTERS, 2022, 120 (23)