Modification of Renewable Cardanol onto Carbon Fiber for the Improved Interfacial Properties of Advanced Polymer Composites

被引：112
作者：
Zheng, Yawen [1 ]
Chen, Lei [2 ]
Wang, Xiaoyun [1 ]
Wu, Guangshun [1 ]
机构：
[1] Ludong Univ, Sch Chem & Mat Sci, Yantai 264025, Peoples R China
[2] Southwest Univ, Coll Text & Garments, Chongqing 400715, Peoples R China
来源：
POLYMERS | 2020年 / 12卷 / 01期
关键词：
carbon fibers; polymer-based composites; fiber-matrix interface; cardanol; surface grafting; REINFORCED EPOXY COMPOSITES; SILICONE RESIN COMPOSITES; MECHANICAL-PROPERTIES; STRENGTH; POLYETHYLENEIMINE; NANOPARTICLES; ENHANCEMENT; ADHESION; SURFACE;
D O I：
10.3390/polym12010045
中图分类号：
O63 [高分子化学（高聚物）];
学科分类号：
070305 ; 080501 ; 081704 ;
摘要：
A facile in situ polymerization was developed for grafting renewable cardanol onto the carbon fiber (CF) surfaces to strengthen the fiber-matrix interface. CFs were chemically modified with hydroxyl groups by using an aryl diazonium reaction, and then copolymerized in situ with hexachlorocyclotriphosphazene (HCCP) and cardanol to build cardanol-modified fibers (CF-cardanol). The cardanol molecules were successfully introduced, as confirmed using Raman spectra and X-ray photoelectron spectroscopy (XPS); the cardanol molecules were found to increase the surface roughness, energy, interfacial wettability, and activity with the matrix resin. As a result, the interlaminar shear strength (ILSS) of CF-cardanol composites increased from 48.2 to 68.13 MPa. In addition, the anti-hydrothermal ageing properties of the modified composites were significantly increased. The reinforcing mechanisms of the fiber-matrix interface were also studied.
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页数：11
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