Non-thermal plasma treatment of Radix aconiti wastewater generated by traditional Chinese medicine processing

被引:12
|
作者
Wen, Yiyong [1 ]
Yi, Jianping [2 ]
Zhao, Shen [1 ]
Jiang, Song [3 ]
Chi, Yuming [2 ]
Liu, Kefu [1 ]
机构
[1] Fudan Univ, Inst Elect Light Sources, Shanghai 200433, Peoples R China
[2] Inst Tong Ren Tang, Beijing 100079, Peoples R China
[3] Univ Shanghai Sci & Technol, Dept Elect Engn, Shanghai 200093, Peoples R China
来源
JOURNAL OF ENVIRONMENTAL SCIENCES | 2016年 / 44卷
基金
中国国家自然科学基金;
关键词
Traditional Chinese medicine (TCM); wastewater; Plasma; Advanced oxidation processes (AOPs); Acute toxicity; Aconitum alkaloid removal; DIELECTRIC BARRIER DISCHARGE; DISRUPTING CHEMICALS EDCS; PULSED CORONA DISCHARGE; METHYLENE-BLUE; PHOTOCATALYTIC DEGRADATION; TOXICITY CHANGE; TEXTILE DYES; GAS; ALKALOIDS; MECHANISM;
D O I
10.1016/j.jes.2015.10.028
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The wastewater effluent from Radix aconiti processing, an important step in the production processes of traditional Chinese medicine (TCM), is a type of toxic wastewater and difficult to treat. Plasma oxidation methods have emerged as feasible techniques for effective decomposition of toxic organic pollutants. This study examined the performance of a plasma reactor operated in a dielectric barrier discharge (DBD) to degrade the effluent from R. aconiti processing. The effects of treatment time, discharge voltage, initial pH value and the feeding gas for the reactor on the degradation of this TCM wastewater were investigated. A bacterium bioluminescence assay was adopted in this study to test the toxicity of the TCM wastewater after non-thermal plasma treatment. The degradation ratio of the main toxic component was 87.77% after 60 min treatment with oxygen used as feed gas and it was 99.59% when the initial pH value was 8.0. High discharge voltage and alkaline solution environment were beneficial for improving the degradation ratio. The treatment process was found to be capable of reducing the toxicity of the wastewater to a low level or even render it non-toxic. These experimental results suggested that the DBD plasma method may be a competitive technology for primary decomposition of biologically undegradable toxic organic pollutants in TCM wastewater. (C) 2016 The Research Center for Eco-=Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B. V.
引用
收藏
页码:99 / 108
页数:10
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