共 49 条
Solution-processable antimony-based light-absorbing materials beyond lead halide perovskites
被引:185
作者:

Boopathi, Karunakara Moorthy
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Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Karuppuswamy, Priyadharsini
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Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan
Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 30013, Taiwan
Natl Tsing Hua Univ, Acad Sinica, Taiwan Int Grad Program, Nano Sci & Technol, Hsinchu, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Singh, Anupriya
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Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Hanmandlu, Chintam
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Chang Gung Univ, Coll Engn, Taoyuan, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Lin, Lin
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Guangxi Univ, Coll Mech Engn, 100,Daxue Dong Rd, Nanning 530004, Peoples R China Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

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Chang, Chien Cheng
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Natl Taiwan Univ, Inst Appl Mech, Roosevelt Rd, Taipei 106, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Wang, Pen Cheng
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Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 30013, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Li, Gang
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Hong Kong Polytech Univ, Dept Elect & Informat Engn, Kowloon, Hong Kong, Peoples R China Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan

Chu, Chih Wei
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Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan
Chang Gung Univ, Coll Engn, Taoyuan, Taiwan Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan
机构:
[1] Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan
[2] Natl Tsing Hua Univ, Dept Engn & Syst Sci, Hsinchu 30013, Taiwan
[3] Natl Tsing Hua Univ, Acad Sinica, Taiwan Int Grad Program, Nano Sci & Technol, Hsinchu, Taiwan
[4] Chang Gung Univ, Coll Engn, Taoyuan, Taiwan
[5] Guangxi Univ, Coll Mech Engn, 100,Daxue Dong Rd, Nanning 530004, Peoples R China
[6] Natl Taiwan Univ, Inst Appl Mech, Roosevelt Rd, Taipei 106, Taiwan
[7] Hong Kong Polytech Univ, Dept Elect & Informat Engn, Kowloon, Hong Kong, Peoples R China
关键词:
SOLAR-CELLS;
THIN-FILMS;
TRANSPORT;
LENGTHS;
CS3SB2I9;
LAYERS;
FIELD;
D O I:
10.1039/c7ta06679a
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Organic-inorganic lead halide perovskites have recently emerged as highly competitive light absorbing materials for low cost solution-processable photovoltaic devices. With the high efficiency already achieved, removing the toxicity, i.e., lead-free and stability are the key obstacles for perovskite solar cells. Here, we report the synthesis of an antimony (Sb)-based hybrid material having the composition of A(3)Sb(2)I(9) [A = CH3NH3 (MA), Cs] and an investigation of its potential photovoltaic applications. Sb-based perovskite-like materials exhibited attractive absorbance properties, with the band gaps of MA(3)Sb(2)I(9) and Cs3Sb2I9 measured to be 1.95 and 2.0 eV, respectively. X-ray photoelectron spectroscopy confirmed the formation of stoichiometric perovskites from appropriate precursor molar ratios incorporated with hydroiodic acid (HI). Planar hybrid Sb-based solar cells exhibited negligible hysteresis and reproducible power output under working conditions. A power conversion efficiency of 2.04% was achieved by the MA(3)Sb(2)I(9) perovskite-based device-the highest reported to date for a Sb-based perovskite solar cell.
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收藏
页码:20843 / 20850
页数:8
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机构:
Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England

Friend, Richard H.
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Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England
[10]
Electron-hole diffusion lengths > 175 μm in solution-grown CH3NH3PbI3 single crystals
[J].
Dong, Qingfeng
;
Fang, Yanjun
;
Shao, Yuchuan
;
Mulligan, Padhraic
;
Qiu, Jie
;
Cao, Lei
;
Huang, Jinsong
.
SCIENCE,
2015, 347 (6225)
:967-970

Dong, Qingfeng
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Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA

Fang, Yanjun
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Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA

Shao, Yuchuan
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Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA

Mulligan, Padhraic
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Ohio State Univ, Dept Mech & Aerosp Engn, Nucl Engn Program, Columbus, OH 43210 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA

Qiu, Jie
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Ohio State Univ, Dept Mech & Aerosp Engn, Nucl Engn Program, Columbus, OH 43210 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA

Cao, Lei
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Ohio State Univ, Dept Mech & Aerosp Engn, Nucl Engn Program, Columbus, OH 43210 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA

Huang, Jinsong
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Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA