Advancing greenhouse gas emission factors for municipal wastewater treatment plants in China

被引:38
作者
Hua, Hui [1 ]
Jiang, Songyan [2 ]
Yuan, Zengwei [1 ]
Liu, Xuewei [1 ]
Zhang, You [1 ]
Cai, Zican [1 ]
机构
[1] Nanjing Univ, Sch Environm, State Key Lab Pollut Control & Resource Reuse, Nanjing 210023, Peoples R China
[2] Nanjing Univ Informat Sci & Technol, Sch Management Sci & Engn, Nanjing 210044, Peoples R China
基金
美国国家科学基金会;
关键词
Carbon emissions; Methane; Nitrous oxide; Carbon dioxide; Climate change; Global warming; NITROUS-OXIDE EMISSIONS; BIOLOGICAL NUTRIENT REMOVAL; ACTIVATED-SLUDGE SYSTEM; N2O EMISSIONS; METHANE EMISSIONS; CONSTRUCTED WETLANDS; NITRIC-OXIDE; SCALE; QUANTIFICATION; A(2)O;
D O I
10.1016/j.envpol.2021.118648
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Estimations of greenhouse gas (GHG) emissions from municipal wastewater treatment plants (MWTPs) remain significant uncertainties in China owing to a lack of reliable emission factors (EFs). This study developed a framework to obtain multi-level (technology, province, and nation) GHG EFs of MWTPs using a database containing 3107 MWTPs in China and published site-specific monitoring data. Results show that GHG EFs of different technologies range widely from 180.0 to 615.7 g CO2-eq/t wastewater, and significant differences are also observed among different provinces in China (190.5-600.3 g CO2-eq/t wastewater), which are generally lower than the previous estimates. It confirms the importance of more detailed technology classification and considering the technological disparity of different provinces in refining GHG estimations of MWTPs. To test the feasibility of the developed EFs, we compared GHG emissions from MWTPs based on multi-level EFs at different spatial and temporal scales. Similar estimation results imply that selecting corresponding EF depending on the availability of activity data would simplify GHG estimations of MWTPs without sacrificing much accuracy. This study contributes a set of well-developed EFs to improve the estimates of GHG emissions from MWTPs, and also offers a method to develop GHG EFs for other sectors.
引用
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页数:10
相关论文
共 90 条
[1]   Methane Emissions from Aerated Zones in a Full-Scale Nitrifying Activated Sludge Treatment Plant [J].
Aboobakar, Amina ;
Jones, Mark ;
Vale, Peter ;
Cartmell, Elise ;
Dotro, Gabriela .
WATER AIR AND SOIL POLLUTION, 2014, 225 (01)
[2]   Nitrous oxide emissions and dissolved oxygen profiling in a full-scale nitrifying activated sludge treatment plant [J].
Aboobakar, Amina ;
Cartmell, Elise ;
Stephenson, Tom ;
Jones, Mark ;
Vale, Peter ;
Dotro, Gabriela .
WATER RESEARCH, 2013, 47 (02) :524-534
[3]   N2O Emissions from Activated Sludge Processes, 2008-2009: Results of a National Monitoring Survey in the United States [J].
Ahn, Joon Ho ;
Kim, Sungpyo ;
Park, Hongkeun ;
Rahm, Brian ;
Pagilla, Krishna ;
Chandran, Kartik .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2010, 44 (12) :4505-4511
[4]  
[Anonymous], 2011, THESIS NANJING U INF
[5]  
[Anonymous], 2013, GETTING EVERY TON EM
[6]   Temporal triggers of N2O emissions during cyclical and seasonal variations of a full-scale sequencing batch reactor treating municipal wastewater [J].
Bae, Wo Bin ;
Park, Yongeun ;
Chandran, Kartik ;
Shin, Jingyeong ;
Kang, Sung Bong ;
Wang, Jinhua ;
Kim, Young Mo .
SCIENCE OF THE TOTAL ENVIRONMENT, 2021, 797
[7]   Assessment of greenhouse gas emission from A/O and SBR wastewater treatment plants in Beijing, China [J].
Bao, Zhiyuan ;
Sun, Shichang ;
Sun, Dezhi .
INTERNATIONAL BIODETERIORATION & BIODEGRADATION, 2016, 108 :108-114
[8]   N2O emissions from full-scale nitrifying biofilters [J].
Bollon, Julien ;
Filali, Ahlem ;
Fayolle, Yannick ;
Guerin, Sabrina ;
Rocher, Vincent ;
Gillot, Sylvie .
WATER RESEARCH, 2016, 102 :41-51
[9]   Comparison of N2O Emissions and Gene Abundances between Wastewater Nitrogen Removal Systems [J].
Brannon, Elizabeth Quinn ;
Moseman-Valtierra, Serena M. ;
Lancellotti, Brittany V. ;
Wigginton, Sara K. ;
Amador, Jose A. ;
McCaughey, James C. ;
Loomis, George W. .
JOURNAL OF ENVIRONMENTAL QUALITY, 2017, 46 (05) :931-938
[10]   Factors controlling nitrous oxide emissions from a full-scale activated sludge system in the tropics [J].
Brotto, Ariane C. ;
Kligerman, Debora C. ;
Andrade, Samara A. ;
Ribeiro, Renato P. ;
Oliveira, Jaime L. M. ;
Chandran, Kartik ;
de Mello, William Z. .
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2015, 22 (15) :11840-11849