共 33 条
Temperature dependence of magnetic excitations in the frustrated antiferromagnetic spinel ZnMn2O
被引:9
作者:

Chang, Hun
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机构:
Korea Univ, Dept Phys, Seoul 02841, South Korea Korea Univ, Dept Phys, Seoul 02841, South Korea

Hwang, In-Yong
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机构:
Korea Univ, Dept Phys, Seoul 02841, South Korea Korea Univ, Dept Phys, Seoul 02841, South Korea

Chung, Jae-Ho
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Korea Univ, Dept Phys, Seoul 02841, South Korea Korea Univ, Dept Phys, Seoul 02841, South Korea

Stewart, J. Ross
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机构:
ISIS Facil, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England Korea Univ, Dept Phys, Seoul 02841, South Korea

Higemoto, Wataru
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机构:
Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan
Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1520081, Japan Korea Univ, Dept Phys, Seoul 02841, South Korea

Miyake, Yasuhiro
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机构:
High Energy Accelerator Res Org, KEK, Tokai, Ibaraki 3191106, Japan Korea Univ, Dept Phys, Seoul 02841, South Korea
机构:
[1] Korea Univ, Dept Phys, Seoul 02841, South Korea
[2] ISIS Facil, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England
[3] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan
[4] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1520081, Japan
[5] High Energy Accelerator Res Org, KEK, Tokai, Ibaraki 3191106, Japan
基金:
新加坡国家研究基金会;
关键词:
LATTICES;
PHASE;
D O I:
10.1103/PhysRevB.97.014406
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
We report the temperature-dependent evolution of spin ordering and excitations of the frustrated tetragonal (c >a) spinel ZnMn2O4 across the two-dimensional antiferromagnetic transition. Muon spin relaxation indicates full development of ordered magnetic moments immediately below T-N = 62.7(2) K in spite of the apparent low-dimensional ordering. Using inelastic neutron scattering, we obtained the spin Hamiltonian accounting for the temperature-dependent spin excitations. The damped spin waves at high temperature exhibit a continuous increase in their lifetime on cooling across T-N. In contrast, the finite anisotropy gap appears suddenly below T-N indicating that single-ion anisotropy stabilizes the antiferromagnetic chains. We also observed the frustrated out-of-plane exchange contributing to the high-energy modes.
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