Tunable photoluminescence of CsPbBr3 perovskite quantum dots for light emitting diodes application

被引:42
作者
Chen, Weiwei [1 ]
Xin, Xing [2 ]
Zang, Zhigang [1 ]
Tang, Xiaosheng [1 ]
Li, Cunlong [1 ]
Hu, Wei [1 ]
Zhou, Miao [1 ]
Du, Juan [2 ]
机构
[1] Chongqing Univ, Key Lab Optoelect Technol & Syst, Minist Educ, Chongqing 400044, Peoples R China
[2] Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, State Key Lab High Field Laser Phys, Shanghai 201800, Peoples R China
基金
中国国家自然科学基金;
关键词
CsPbBr3; Photoluminescence; Blinking; Lifetime; Light emitting diodes; CESIUM LEAD HALIDE; SINGLE-PHOTON EMISSION; SOLAR-CELLS; NANOCRYSTALS; EXCHANGE; CSPBX3; NANOWIRES; BLINKING; BR; CL;
D O I
10.1016/j.jssc.2017.06.006
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
All-inorganic cesium lead halide (CsPbBr3) perovskite quantum dots (QDs), as one kind of promising materials, have attracted considerable attention in optoelectronic applications. Herein, we synthesized the colloidal CsPbBr3 QDs with tunable photoluminescence (PL) (493-531 nm) by adjusting the reaction temperatures, which revealed narrow emission bandwidths of about 25 nm. The average diameters of the QDs could be adjusted from 7.1 to 12.3 nm as the temperature increased from 100 degrees C to 180 degrees C. Moreover, the radiative lifetimes of CsPbBr3 QDs were measured to be similar to 2 ns, and the single QD fluorescence intensity time trace results demonstrated its suppressed blinking emission. Moreover, green light emitting diodes by using CsPbBr3 QDs tasted on blue LED chips were further fabricated, which provided potential applications in the field of display and lighting technology.
引用
收藏
页码:115 / 120
页数:6
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