Tunable photoluminescence of CsPbBr3 perovskite quantum dots for light emitting diodes application

被引:40
作者
Chen, Weiwei [1 ]
Xin, Xing [2 ]
Zang, Zhigang [1 ]
Tang, Xiaosheng [1 ]
Li, Cunlong [1 ]
Hu, Wei [1 ]
Zhou, Miao [1 ]
Du, Juan [2 ]
机构
[1] Chongqing Univ, Key Lab Optoelect Technol & Syst, Minist Educ, Chongqing 400044, Peoples R China
[2] Chinese Acad Sci, Shanghai Inst Opt & Fine Mech, State Key Lab High Field Laser Phys, Shanghai 201800, Peoples R China
基金
中国国家自然科学基金;
关键词
CsPbBr3; Photoluminescence; Blinking; Lifetime; Light emitting diodes; CESIUM LEAD HALIDE; SINGLE-PHOTON EMISSION; SOLAR-CELLS; NANOCRYSTALS; EXCHANGE; CSPBX3; NANOWIRES; BLINKING; BR; CL;
D O I
10.1016/j.jssc.2017.06.006
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
All-inorganic cesium lead halide (CsPbBr3) perovskite quantum dots (QDs), as one kind of promising materials, have attracted considerable attention in optoelectronic applications. Herein, we synthesized the colloidal CsPbBr3 QDs with tunable photoluminescence (PL) (493-531 nm) by adjusting the reaction temperatures, which revealed narrow emission bandwidths of about 25 nm. The average diameters of the QDs could be adjusted from 7.1 to 12.3 nm as the temperature increased from 100 degrees C to 180 degrees C. Moreover, the radiative lifetimes of CsPbBr3 QDs were measured to be similar to 2 ns, and the single QD fluorescence intensity time trace results demonstrated its suppressed blinking emission. Moreover, green light emitting diodes by using CsPbBr3 QDs tasted on blue LED chips were further fabricated, which provided potential applications in the field of display and lighting technology.
引用
收藏
页码:115 / 120
页数:6
相关论文
共 28 条
  • [1] Highly Luminescent Colloidal Nanoplates of Perovskite Cesium Lead Halide and Their Oriented Assemblies
    Bekenstein, Yehonadav
    Koscher, Brent A.
    Eaton, Samuel W.
    Yang, Peidong
    Alivisatos, A. Paul
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2015, 137 (51) : 16008 - 16011
  • [2] Composition-Dependent Hot Carrier Relaxation Dynamics in Cesium Lead Halide (CsPbX3, X = Br and I) Perovskite Nanocrystals
    Chung, Heejae
    Jung, Seok Il
    Kim, Hyo Jin
    Cha, Wonhee
    Sim, Eunji
    Kim, Dongho
    Koh, Weon-Kyu
    Kim, Jiwon
    [J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2017, 56 (15) : 4160 - 4164
  • [3] All-solid-state dye-sensitized solar cells with high efficiency
    Chung, In
    Lee, Byunghong
    He, Jiaqing
    Chang, Robert P. H.
    Kanatzidis, Mercouri G.
    [J]. NATURE, 2012, 485 (7399) : 486 - U94
  • [4] Universal emission intermittency in quantum dots, nanorods and nanowires
    Frantsuzov, Pavel
    Kuno, Masaru
    Janko, Boldizsar
    Marcus, Rudolph A.
    [J]. NATURE PHYSICS, 2008, 4 (07) : 519 - 522
  • [5] Control of Emission Color of High Quantum Yield CH3 NH3 PbBr3 Perovskite Quantum Dots by Precipitation Temperature
    Huang, He
    Susha, Andrei S.
    Kershaw, Stephen V.
    Hung, Tak Fu
    Rogach, Andrey L.
    [J]. ADVANCED SCIENCE, 2015, 2 (09)
  • [6] Reversible Halide Exchange Reaction of Organometal Trihalide Perovskite Colloidal Nanocrystals for Full-Range Band Gap Tuning
    Jang, Dong Myung
    Park, Kidong
    Kim, Duk Hwan
    Park, Jeunghee
    Shojaei, Fazel
    Kang, Hong Seok
    Ahn, Jae-Pyung
    Lee, Jong Woon
    Song, Jae Kyu
    [J]. NANO LETTERS, 2015, 15 (08) : 5191 - 5199
  • [7] Kaltenbrunner M, 2015, NAT MATER, V14, P1032, DOI [10.1038/NMAT4388, 10.1038/nmat4388]
  • [8] Highly pure green light emission of perovskite CsPbBr3 quantum dots and their application for green light-emitting diodes
    Li, Cunlong
    Zang, Zhigang
    Chen, Weiwei
    Hu, Zhiping
    Tang, Xiaosheng
    Hu, Wei
    Sun, Kuan
    Liu, Xianming
    Chen, Weimin
    [J]. OPTICS EXPRESS, 2016, 24 (13): : 15071 - 15078
  • [9] McGehee MD, 2014, NAT MATER, V13, P845, DOI 10.1038/nmat4050
  • [10] Fast Anion-Exchange in Highly Luminescent Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, I)
    Nedelcu, Georgian
    Protesescu, Loredana
    Yakunin, Sergii
    Bodnarchuk, Maryna I.
    Grotevent, Matthias J.
    Kovalenko, Maksym V.
    [J]. NANO LETTERS, 2015, 15 (08) : 5635 - 5640