Numerical analysis of the influence of the channel cross-section aspect ratio on the performance of a PEM fuel cell with serpentine flow field design

被引:102
作者
Manso, A. P. [1 ]
Marzo, F. F. [2 ]
Garmendia Mujika, M. [1 ]
Barranco, J. [3 ]
Lorenzo, A. [2 ]
机构
[1] Univ Basque Country, Graph Express & Engn Projects Dept, San Sebastian, Spain
[2] Univ Basque Country, Chem Engn & Environm Dept, San Sebastian, Spain
[3] Univ Zaragoza, Dept Mech Engn, Zaragoza, Spain
关键词
PEMFC; Fuel cell; Flow-field design; Simulation; es-pemfc; Aspect ratio; CURRENT DISTRIBUTIONS; WATER; PLATES; RIB;
D O I
10.1016/j.ijhydene.2011.02.099
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This work numerically investigates the influence of the channel cross-section aspect ratio (defined as the ratio height/width) on the performance of a PEM fuel cell with serpentine flow field (SFF) design. The local current densities, velocity distributions, liquid water concentration in the membrane, hydrogen and oxygen concentrations and temperature were analyzed in the PEM fuel cell for 10 different aspect ratios, varying between 0.07 and 15, to understand the channel cross-section aspect ratio effect. Tie area of the channel cross section (1.06 mm(2)) and the total effective reactive area of the PEM fuel cell (256 mm(2)) were maintained constant in all cases. The obtained results show that at low operating voltages the cell performance is independent of the channel cross-section aspect ratio. At high operating voltages, where the influence of mass transporting velocity is predominant, as the channel cross-section aspect ratio increases the cell performance is improved. The models with high aspect ratio show, in general, more uniform current distributions, with the higher maximum and minimum intensity values, temperature distributions with smaller gradients and a superior contain of water in the membrane, which allows to obtain a higher performance. From these models the 10/06 and 12/05 aspect ratio present the best combination of variables, as shown by their polarization curves. Copyright (C) 2011, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:6795 / 6808
页数:14
相关论文
共 24 条
[1]  
[Anonymous], ES PEMFC METH TUT MA
[2]   Operating proton exchange membrane fuel cells without external humidification of the reactant gases - Fundamental aspects [J].
Buchi, FN ;
Srinivasan, S .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1997, 144 (08) :2767-2772
[3]   Investigation of the transversal water profile in nafion membranes in polymer electrolyte fuel cells [J].
Büchi, FN ;
Scherer, GG .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2001, 148 (03) :A183-A188
[4]   The scaling behavior of flow patterns: a model investigation [J].
Cha, SW ;
O'Hayre, R ;
Saito, Y ;
Prinz, FB .
JOURNAL OF POWER SOURCES, 2004, 134 (01) :57-71
[5]   Numerical studies on the geometrical characterization of serpentine flow-field for efficient PEMFC [J].
Choi, Kap-Seung ;
Kim, Hyung-Man ;
Moon, Sung-Mo .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2011, 36 (02) :1613-1627
[6]   On the relative influence of convection in serpentine flow fields of PEM fuel cells [J].
Feser, J. P. ;
Prasad, A. K. ;
Advani, S. G. .
JOURNAL OF POWER SOURCES, 2006, 161 (01) :404-412
[7]  
Hoogers G., 2003, Fuel Cells Technology Handbook, V1st, p1
[8]   The effect of serpentine flow-field designs on PEM fuel cell performance [J].
Jeon, D. H. ;
Greenway, S. ;
Shimpalee, S. ;
Van Zee, J. W. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2008, 33 (03) :1052-1066
[9]   Parametric study of the channel design at the bipolar plate in PEMFC performances [J].
Lee, Sungho ;
Jeong, Heeseok ;
Ahn, Byungki ;
Lim, Taewon ;
Son, Youngiin .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2008, 33 (20) :5691-5696
[10]   Verifying predictions of water and current distributions in a serpentine flow field polymer electrolyte membrane fuel cell [J].
Lee, WK ;
Shimpalee, S ;
Van Zee, JW .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2003, 150 (03) :A341-A348