Detecting the out-of-time-order correlations of dynamical quantum phase transitions in a solid-state quantum simulator

Quantum many-body systems in equilibrium can be effectively characterized using the framework of quantum statistical mechanics. However, there still exist a lot of questions regarding how to understand the nonequilibrium dynamical behavior of quantum many-body systems, which are not accessible with the thermodynamic description. Experiments in quantum simulators are opening up a route toward the generation of quantum states beyond the equilibrium paradigm. As an example, in closed quantum many-body systems, dynamical quantum phase transitions act as phase transitions in time, with physical quantities becoming nonanalytic at a critical time, extending important principles such as universality to the nonequilibrium realm. Here, in a solid-state quantum simulator, we report the experimental detection of out-of-time-order correlators in the presence of nonequilibrium phase transitions with the transverse field Ising model, which are a central concept to quantify quantum information scrambling and quantum chaos. Through measuring the multiple quantum spectra, we eventually observe the buildup of quantum correlation. Further applications of this protocol could potentially enable studies of other exotic phenomena such as many-body localization and tests of the holographic duality between quantum and gravitational systems.