Assembly of Two Self-Interpenetrating Metal-Organic Frameworks Based on a Trigonal Ligand: Syntheses, Crystal Structures, and Properties

被引：29
作者：
Guo, Feng [1 ]
Su, Changhua [3 ]
Fan, Yuhang [1 ]
Shi, Wenbing [1 ]
Zhang, Xiuling [2 ]
机构：
[1] Yangtze Normal Univ, Chongqing Key Lab Inorgan Special Funct Mat, Coll Chem & Chem Engn, Chongqing 408100, Peoples R China
[2] Dezhou Univ, Coll Chem & Chem Engn, Dezhou 253023, Peoples R China
[3] Liaocheng Univ, Sch Mat Sci & Engn, Liaocheng 252059, Shandong, Peoples R China
来源：
INORGANIC CHEMISTRY | 2020年 / 59卷 / 10期
关键词：
RESPONSIVE LUMINESCENT SENSOR; LEWIS BASIC SITES; KNOEVENAGEL CONDENSATION REACTION; EFFICIENT HETEROGENEOUS CATALYST; SELECTIVE GAS-ADSORPTION; SOLVENT-FREE CATALYST; CHEMICAL TRANSFORMATION; SINGLE-CRYSTAL; CO2; MOF;
D O I：
10.1021/acs.inorgchem.0c00596
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Two self-interpenetrating metal-organic frameworks (MOFs) 1 and 2 were designed and constructed through the coordination self-assembly of transition metal nodes and a trigonal ligand. They both exhibit interesting three-dimensional constructions with the 1 + 2 self-locked mode. Because of the outstanding moisture susceptibility and luminescence property, MOF 1 has a potential detectability toward nitrofurantoin (NFT) in water. More importantly, MOF 1 can efficiently monitor NFT in bovine serum. Taking into account of Lewis basic sites in the skeleton, MOF 2 can be implemented as an outstanding heterogeneous catalyst for the Knoevenagel reaction. Furthermore, they both reveal excellent circularity and an application effect for five cycles.
引用
收藏
页码：7135 / 7142
页数：8
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