Many-body dipole-dipole interactions between excited Rb atoms probed by wave packets and parametric four-wave mixing

被引:17
作者
Shen, F. [1 ]
Gao, J. [1 ]
Senin, A. A. [1 ]
Zhu, C. J. [1 ]
Allen, J. R. [1 ]
Lu, Z. H. [1 ]
Xiao, Y. [1 ]
Eden, J. G. [1 ]
机构
[1] Univ Illinois, Dept Elect & Comp Engn, Lab Opt Phys & Engn, Urbana, IL 61801 USA
关键词
D O I
10.1103/PhysRevLett.99.143201
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Dipole-dipole interactions between excited Rb atoms at long range (similar to 300a(0)-2150a(0)) have been observed with molecular wave packets and a coherent nonlinear optical process. Fourier analysis of the parametric four-wave mixing (PFWM) signal wave intensity produced in femtosecond pump-probe experiments demonstrates the appearance of sidebands associated with the Rb 7s-5d(5/2) quantum beating frequency of similar to 18.3 THz. Calculations show that the observed sideband splittings and Fourier domain profiles result from multiple atom, dipole-dipole interactions, and ensembles comprising five or fewer Rb (7s, 6p) atoms account for virtually all of the data.
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页数:4
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