Spatial distribution of particulate matter on winter nights in Temuco, Chile: Studying the impact of residential wood-burning using mobile monitoring

被引:11
作者
Blanco, Estela [1 ]
Rubilar, Francisco [2 ]
Quinteros, Maria Elisa [3 ]
Cayupi, Karen [2 ]
Ayala, Salvador [1 ]
Lu, Siyao [4 ]
Jimenez, Raquel B. [5 ]
Blazquez, Carola A. [6 ]
Delgado-Saborit, Juana Maria [7 ,8 ]
Harrison, Roy M. [7 ,9 ]
Ruiz-Rudolph, Pablo [10 ]
Cardenas, Juan Pablo [2 ]
机构
[1] Univ Chile, Fac Med, Programa Doctorado Salud Publ, Inst Salud Poblac, Independencia 939, Santiago, Chile
[2] Univ La Frontera, Inst Medio Ambiente, Ave Francisco Salazar, Temuco 01145, Chile
[3] Univ Talca, Fac Ciencias Salud, Dept Salud Publ, Ave Lircay S-N, Talca, Chile
[4] Univ Michigan, Dept Environm Hlth Sci, 1415 Washington Hts, Ann Arbor, MI 48109 USA
[5] Boston Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA USA
[6] Univ Andres Bello, Dept Engn Sci, 980 Quillota, Vina Del Mar 2531015, Chile
[7] Univ Birmingham, Sch Geog Earth & Environm Sci, Div Environm Hlth & Risk Management, Birmingham, England
[8] Univ Jaume 1, Sch Med, Perinatal Epidemiol Environm Hlth & Clin Res, Avinguda de Vicent Sos Baynat S-N, Castellon De La Plana 12071, Castellon, Spain
[9] King Abdulaziz Univ, Ctr Excellence Environm Studies, Dept Environm Sci, POB 80203, Jeddah 21589, Saudi Arabia
[10] Univ Chile, Fac Med, Programa Salud Ambiental, Inst Salud Poblac, Independencia 939, Santiago, Chile
关键词
Air pollution; Air quality; Wood smoke; Global positioning system; Mobile sampling; AIR-POLLUTION; ULTRAFINE PARTICLES; PM2.5; SANTIAGO; VARIABILITY; EMISSIONS; MODEL; CITY; COMBUSTION; POLLUTANTS;
D O I
10.1016/j.atmosenv.2022.119255
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Temuco, a medium-sized city in the south of Chile, is heavily impacted by residential wood-burning particularly in winter, which causes strong episodes of air pollution. We spatially characterized the distribution of particulate matter (PM) during winter nights in Temuco using mobile measurements. In winter 2016 (June 8-July 15th), continuous monitors for PM <= 2.5 mu m (PM2.5) and ultrafine particles <0.1 mu m (UFP) were deployed in a vehicle along with a positioning system during 20 nights (20:00 to 2:00) in assigned routes that crossed the city and additional sampling was conducted at a central site. Measurements were expressed as concentrations and ratios to central site concentrations and collapsed by spatial grids of 50, 100, 200, and 400 m. Average PM2.5 concentrations were similar to 100 mu g m(-3), while UFP similar to 30,000 counts cm(-3). Some neighborhoods had concentrations of PM2.5 nearly double those measured at a centrally located site, while other neighborhoods had less than half the measured level. We identified hotspots and cold spots of PM2.5 and UFP throughout the urban area-and observed some neighborhoods in which over 20% of the area was categorized as a hotspot for one of the pollutants (14 for PM2.5 and 11 for UFP out of 34). Using mobile monitoring-a relatively simple and inexpensive methodology-we characterized the spatial distribution of pollutants and likely clusters for the time period, which may guide future spatial campaigns and help targeting local interventions aimed at air pollution mitigation.
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页数:10
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