Radiochemical separations and experimental measurements of short-lived fission products from 14 MeV irradiation of depleted uranium

被引:6
作者
Arrigo, Leah M. [1 ]
Greenwood, Lawrence R. [1 ]
Pierson, Bruce D. [1 ]
Metz, Lori A. [1 ]
Friese, Judah I. [1 ]
机构
[1] Pacific Northwest Natl Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA
关键词
Radiochemical separations; Fission products; Short-lived radionuclides; Actinide fission; 14 MeV fission; YIELDS;
D O I
10.1007/s10967-018-6115-7
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
This work focused on the experimental analysis of depleted uranium irradiated with 14 MeV neutrons to obtain fission yields for 20 fission products with half-lives ranging from 16.8 h to 30.1 years. Several analytes were identified where improvements to the available nuclear data would be beneficial. The results obtained from this experiment could be used to make improvements to cumulative fission yield data once confirmatory measurements are made. The required separations will be described along with a comparison to the reported Evaluated Nuclear Data File fission yields and other experimental measurements.
引用
收藏
页码:353 / 360
页数:8
相关论文
共 16 条
  • [1] ADAIR HL, 1975, NUCL TECHNOL, V25, P224, DOI 10.13182/NT75-A24365
  • [2] ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data
    Chadwick, M. B.
    Herman, M.
    Oblozinsky, P.
    Dunn, M. E.
    Danon, Y.
    Kahler, A. C.
    Smith, D. L.
    Pritychenko, B.
    Arbanas, G.
    Arcilla, R.
    Brewer, R.
    Brown, D. A.
    Capote, R.
    Carlson, A. D.
    Cho, Y. S.
    Derrien, H.
    Guber, K.
    Hale, G. M.
    Hoblit, S.
    Holloway, S.
    Johnson, T. D.
    Kawano, T.
    Kiedrowski, B. C.
    Kim, H.
    Kunieda, S.
    Larson, N. M.
    Leal, L.
    Lestone, J. P.
    Little, R. C.
    McCutchan, E. A.
    MacFarlane, R. E.
    MacInnes, M.
    Mattoon, C. M.
    McKnight, R. D.
    Mughabghab, S. F.
    Nobre, G. P. A.
    Palmiotti, G.
    Palumbo, A.
    Pigni, M. T.
    Pronyaev, V. G.
    Sayer, R. O.
    Sonzogni, A. A.
    Summers, N. C.
    Talou, P.
    Thompson, I. J.
    Trkov, A.
    Vogt, R. L.
    van der Marck, S. C.
    Wallner, A.
    White, M. C.
    [J]. NUCLEAR DATA SHEETS, 2011, 112 (12) : 2887 - 2996
  • [4] Separation and quantification of chemically diverse analytes in neutron irradiated fissile materials
    Douglas, M.
    Friese, J. I.
    Greenwood, L. R.
    Farmer, O. T., III
    Thomas, M. L.
    Maiti, T. C.
    Finn, E. C.
    Garofoli, S. J.
    Gassman, P. L.
    Huff, M. M.
    Schulte, S. M.
    Smith, S. C.
    Thomas, K. K.
    Bachelor, P. P.
    [J]. JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2009, 282 (01) : 63 - 68
  • [5] Short-lived fission product measurements from >0.1 MeV neutron-induced fission using boron carbide
    Finn, Erin
    Metz, Lori
    Greenwood, Larry
    Pierson, Bruce
    Friese, Judah
    Kephart, Rosara
    Kephart, Jeremy
    [J]. JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2012, 293 (01) : 267 - 272
  • [6] Cumulative fission yields of short-lived isotopes under natural-abundance-boron-carbide-moderated neutron spectrum
    Finn, Erin C.
    Metz, Lori
    Greenwood, Larry
    Pierson, Bruce
    Wittman, Richard
    Friese, Judah
    Kephart, Rosara
    [J]. JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2015, 306 (01) : 79 - 91
  • [7] Energy Dependence of Fission Product Yields from 235U, 238U and 239Pu for Incident Neutron Energies Between 0.5 and 14.8 MeV
    Gooden, M. E.
    Arnold, C. W.
    Becker, J. A.
    Bhatia, C.
    Bhike, M.
    Bond, E. M.
    Bredeweg, T. A.
    Fallin, B.
    Fowler, M. M.
    Howell, C. R.
    Kelley, J. H.
    Krishichayan
    Macri, R.
    Rusev, G.
    Ryan, C.
    Sheets, S. A.
    Stoyer, M. A.
    Tonchev, A. P.
    Tornow, W.
    Vieira, D. J.
    Wilhelmy, J. B.
    [J]. NUCLEAR DATA SHEETS, 2016, 131 : 319 - 356
  • [8] Greenwood LR, 2013, PNNL22253, DOI [10.2172/1067961, DOI 10.2172/1067961]
  • [9] Jackson MJ, 2018, MARC 11 C
  • [10] Measurement of 160Tb and 161Tb in nuclear forensics samples
    Jiang, J.
    Davies, A. V.
    Britton, R. E.
    [J]. JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2017, 314 (02) : 727 - 736