Sensing with Multipolar Second Harmonic Generation from Spherical Metallic Nanoparticles

被引：121

作者：

Butet, Jeremy ^{[1
]}

Russier-Antoine, Isabelle ^{[1
]}

Jonin, Christian ^{[1
]}

Lascoux, Noelle ^{[1
]}

Benichou, Emmanuel ^{[1
]}

Brevet, Pierre-Francois ^{[1
]}

机构：

[1] Univ Lyon 1, UMR CNRS 5579, Lab Spectrometrie Ion & Mol LASIM, F-69622 Villeurbanne, France

来源：

NANO LETTERS | 2012年 / 12卷 / 03期

关键词：

Silver nanoparticles; nonlinear optical sensing; plasmonics; second harmonic generation; CENTROSYMMETRIC MATERIAL; FANO RESONANCE; NANOSTRUCTURES; SPECTROSCOPY; MORPHOLOGY; SPHERES;

D O I：

10.1021/nl300203u

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

We show that sensing in the nonlinear optical regime using multipolar surface plasmon resonances is more sensitive in comparison to sensing in the linear optical regime. Mie theory, and its extension to the second harmonic generation from a metallic nanosphere, is used to describe multipolar second harmonic generation from silver metallic nanoparticles. The standard figure of merit of a potential plasmonic sensor based on this principle is then calculated. We finally demonstrate that such a sensor is more sensitive to optical refraction index changes occurring in the vicinity of the metallic nanoparticle than its linear counterpart.

引用

页码：1697 / 1701

页数：5

共 32 条

[1] Biosensing with plasmonic nanosensors
Anker, Jeffrey N.
Hall, W. Paige
Lyandres, Olga
Shah, Nilam C.
Zhao, Jing
Van Duyne, Richard P.
[J]. NATURE MATERIALS, 2008, 7 (06) : 442 - 453
[2] Origin of optical second-harmonic generation in spherical gold nanoparticles: Local surface and nonlocal bulk contributions
Bachelier, G.
Butet, J.
Russier-Antoine, I.
Jonin, C.
Benichou, E.
Brevet, P-F
[J]. PHYSICAL REVIEW B, 2010, 82 (23)
[3] Fano Profiles Induced by Near-Field Coupling in Heterogeneous Dimers of Gold and Silver Nanoparticles
Bachelier, G.
Russier-Antoine, I.
Benichou, E.
Jonin, C.
Del Fatti, N.
Vallee, F.
Brevet, P. -F.
[J]. PHYSICAL REVIEW LETTERS, 2008, 101 (19)
[4] Multipolar second-harmonic generation in noble metal nanoparticles
Bachelier, Guillaume
Russier-Antoine, Isabelle
Benichou, Emmanuel
Jonin, Christian
Brevet, Pierre-Francois
[J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 2008, 25 (06) : 955 - 960
[5] Optical extinction spectroscopy of single silver nanoparticles
Billaud, P.
Huntzinger, J.-R.
Cottancin, E.
Lerme, J.
Pellarin, M.
Arnaud, L.
Broyer, M.
Del Fatti, N.
Vallee, F.
[J]. EUROPEAN PHYSICAL JOURNAL D, 2007, 43 (1-3) : 271 - 274
[6] Bohren C.F, 2008, Absorption and Scattering of Light by Small Particles
[7] Interference between Selected Dipoles and Octupoles in the Optical Second-Harmonic Generation from Spherical Gold Nanoparticles
Butet, J.
Bachelier, G.
Russier-Antoine, I.
Jonin, C.
Benichou, E.
Brevet, P. -F.
[J]. PHYSICAL REVIEW LETTERS, 2010, 105 (07)
[8] Optical Second Harmonic Generation of Single Metallic Nanoparticles Embedded in a Homogeneous Medium
Butet, Jeremy
Duboisset, Julien
Bachelier, Guillaume
Russier-Antoine, Isabelle
Benichou, Emmanuel
Jonin, Christian
Brevet, Pierre-Francois
[J]. NANO LETTERS, 2010, 10 (05) : 1717 - 1721
[9] Chandra R. P., 2010, CHEM REV, V110, P5332
[10] Second-harmonic Rayleigh scattering from a sphere of centrosymmetric material
Dadap, JI
Shan, J
Eisenthal, KB
Heinz, TF
[J]. PHYSICAL REVIEW LETTERS, 1999, 83 (20) : 4045 - 4048

← 1 2 3 4 →