Enhanced NOx Reduction by Combined Staged Air and Flue Gas Recirculation in Biomass Grate Combustion

被引:47
作者
Houshfar, Ehsan [1 ]
Khalil, Roger A. [2 ]
Lovas, Terese [1 ]
Skreiberg, Oyvind [2 ]
机构
[1] Norwegian Univ Sci & Technol NTNU, Dept Energy & Proc Engn, NO-7491 Trondheim, Norway
[2] SINTEF Energy Res, Dept Thermal Energy, NO-7465 Trondheim, Norway
关键词
COAL COMBUSTION; PULVERIZED COAL; NITRIC-OXIDE; NITROGEN; EMISSIONS; HCN; WOOD; NH3; PYROLYSIS; MECHANISM;
D O I
10.1021/ef300199g
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Flue gas recirculation (FGR) is a conventional means of reducing NOx emissions that involves lowering the peak flame temperature and reducing the oxygen concentration in the combustion region. Staged air combustion is also an effective means of NOx reduction, especially in biomass combustion. This article reports results on NOx emissions in a set of experiments combining FGR and staged air combustion in a grate-fired laboratory-scale reactor. Two different compositions of the recirculated flue gas were used: CO2 and CO2 + NO. The CO2 concentration varied between 0-8 vol % of the total inlet flow rate and the NO concentration varied between 0 and 64 ppm. Two different FGR locations were also tested: above and below the grate. The results are compared with a reference experiment performed without FGR The NOx reduction level from staged air combustion at the optimal primary excess air ratio is similar to 70%, while employing FGR can reduce the NOx emissions by an additional 5%-10%. The optimal primary excess air ratio range is 0.9-1. However, FGR more effectively reduces NOx when employed outside of the optimum primary excess air ratio range, i.e., excess air ratios higher than 1 and less than 0.9. The experiments with FGR located above the grate exhibit higher reduction potential, while FGR located below the grate produces decreased reduction. The recycled-NO conversion factor, which gives a measure of maximal FGR efficiency, at the maximum point, is nearly 100% when FGR is applied below the grate and is 85%-100% in the case of recirculation above the grate.
引用
收藏
页码:3003 / 3011
页数:9
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