Distribution and accumulation of endocrine-disrupting chemicals and pharmaceuticals in wastewater irrigated soils in Hebei, China

被引:207
作者
Chen, Feng [1 ]
Ying, Guang-Guo [1 ]
Kong, Ling-Xiao [2 ]
Wang, Li [1 ]
Zhao, Jian-Liang [1 ]
Zhou, Li-Jun [1 ]
Zhang, Li-Juan [1 ]
机构
[1] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
[2] Hebei Acad Agr & Forestry Sci, Inst Plant Protect, Baoding 07100, Peoples R China
基金
中国国家自然科学基金;
关键词
Endocrine-disrupting chemicals; Pharmaceuticals; Soil; Wastewater; Irrigation; PERSONAL CARE PRODUCTS; TANDEM MASS-SPECTROMETRY; HUDSON RIVER ESTUARY; ENVIRONMENTAL FATE; MICROBIAL ACTIVITY; TREATMENT PLANTS; RECLAIMED WATER; RISK-ASSESSMENT; HEAVY-METALS; SOUTH CHINA;
D O I
10.1016/j.envpol.2011.03.016
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study investigated the occurrence of 43 emerging contaminants including 9 endocrine-disrupting chemicals and 34 pharmaceuticals in three sites in Hebei Province, north China. Each site has a wastewater irrigated plot and a separate groundwater irrigated plot for comparison purpose. The results showed that the concentrations of the target compounds in the wastewater irrigated soils were in most cases higher than those in the groundwater irrigated soils. Among the 43 target compounds, nine compounds bisphenol-A, triclocarban, triclosan, 4-nonylphenol, salicylic acid, oxytetracycline, tetracycline, trimethoprim and primidone were detected at least once in the soils. Preliminary environmental risk assessment showed that triclocarban might pose high risks to terrestrial organisms while the other detected compounds posed minimal risks. Irrigation with wastewater could lead to presence or accumulation of some emerging contaminants to some extent in irrigated soils. (C) 2011 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1490 / 1498
页数:9
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