Field-free molecular orientation by a multicolor laser field

被引:41
|
作者
Zhang, Shian [1 ,2 ]
Shi, Junhui [3 ]
Zhang, Hui [1 ,2 ]
Jia, Tianqing [1 ,2 ]
Wang, Zugeng [1 ,2 ]
Sun, Zhenrong [1 ,2 ]
机构
[1] E China Normal Univ, State Key Lab Precis Spect, Shanghai 200062, Peoples R China
[2] E China Normal Univ, Dept Phys, Shanghai 200062, Peoples R China
[3] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
来源
PHYSICAL REVIEW A | 2011年 / 83卷 / 02期
关键词
ALIGNMENT;
D O I
10.1103/PhysRevA.83.023416
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We theoretically study the field-free molecular orientation by a multicolor laser field with a superposition of the fundamental wave and its harmonics. It is shown that the molecular orientation will be up to a maximum value pumped by the four-color laser field at the same laser intensity, and the molecular orientation direction and its degree can be controlled by varying the carrier-envelope phase of the four-color laser field. It is also indicated that the molecular orientation induced by a four-color laser field can be tremendously enhanced by applying another in-phase or out-phase four-color laser field at the beginning of the rotational wave-packet rephasing or the end of the rotational wave-packet dephasing.
引用
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页数:5
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