Continuous, high-flux and efficient oil/water separation assisted by an integrated system with opposite wettability

被引:66
作者
Li, Jian [1 ]
Long, Yifei [1 ]
Xu, Changcheng [1 ]
Tian, Haifeng [1 ]
Wu, Yanxia [1 ]
Zha, Fei [1 ]
机构
[1] Northwest Normal Univ, Coll Chem & Chem Engn, Lanzhou 730070, Gansu, Peoples R China
基金
中国博士后科学基金;
关键词
Electrodeposition; Two-way separation device; Continuous oil/water separation; Opposite wettability; High separation efficiency; High-flux; SUPEROLEOPHOBIC SURFACES; EMULSION SEPARATION; OIL; WATER; MESH; FABRICATION; MEMBRANES; SUPERWETTABILITY; MIXTURE;
D O I
10.1016/j.apsusc.2017.10.056
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
To resolve the drawbacks that single-mesh involved for oil/water separation, such as batch processing mode, only one phase was purified and the quick decrease in flux et al., herein, a two-way separation T-tube device was designed by integrating a pair of meshes with opposite wettability, i.e., underwater superoleophobic and superhydrophobic/superoleophilic properties. Such integrated system can continuously separate both oil and water phase from the oil/water mixtures simultaneously through one-step procedure with high flux (above 3.675 L m(-2) s(-1)) and high separation efficiency larger than 99.8% regardless of the heavy oil or light oil involved in the mixture. Moreover, the as-prepared two meshes still maintained high separation efficiency larger than above 98.9% even after 50 cycle-usages. It worthy mentioned that this two-way separation mode essentially solves the oil liquid accumulation problem that is the single separation membrane needs to tolerate a large hydrostatic pressure caused by the accumulated liquid. We deeply believe this two-way separation system would provide a new strategy for realizing practical applications in oil spill clean-up via a continuous mode. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:374 / 380
页数:7
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