Effect of the inner liner on the hydrogen distribution of zircaloy-2 nuclear fuel claddings

被引:10
作者
Duarte, Liliana I. [1 ]
Fagnoni, Francesco [1 ,2 ]
Zubler, Robert [1 ]
Gong, Weijia [1 ]
Trtik, Pavel [3 ]
Bertsch, Johannes [1 ]
机构
[1] Paul Scherrer Inst, Lab Nucl Mat, Forsch Str 111, CH-5232 Villigen, Switzerland
[2] Swiss Fed Inst Technol, Dept Mat, Lab Nanomet, Vladimir Prelog Weg 5, CH-8093 Zurich, Switzerland
[3] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, Forsch Str 111, CH-5232 Villigen, Switzerland
关键词
Hydrides; Hydrogen diffusion; Zirconium Cladding alloys; Zry-2; Liner; Neutron Radiography; Neutron Imaging; OXYSULFIDE SCINTILLATOR SCREENS; ZIRCONIUM ALLOYS;
D O I
10.1016/j.jnucmat.2021.153284
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Hydrides precipitation has been induced by slow cooling of hydrogen-charged specimens of three different Zircaloy-2 claddings commonly used in boiling water reactors. The resulting hydrides distribution has been analysed by optical and scanning electron microscopy and neutron radiography. With the latter technique, it is possible to quantify radially the hydrogen concentration with a resolution of +/- 10 wppm and a spatial resolution of 10 mu m. Hydrogenated samples were subjected to a temperature of 400 degrees C and afterwards a cooling rate of 0.3 degrees C/h and 10 degrees C/h showed that practically a complete migration of the hydrogen towards the liner-cladding interface took place, leading to very high local hydrogen concentrations exceeding 2000 wppm. (C) 2021 Elsevier B.V. All rights reserved.
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页数:6
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