Momentum-resolved resonant inelastic soft X-ray scattering (qRIXS) endstation at the ALS

被引：8

作者：

Chuang, Yi-De ^{[1
]}

Feng, Xuefei ^{[1
]}

Cruz, Alejandro ^{[1
]}

Hanzel, Kelly ^{[2
]}

Brown, Adam ^{[2
]}

Spucces, Adrian ^{[2
]}

Frano, Alex ^{[1
,3
]}

Lee, Wei-Sheng ^{[4
]}

Kim, Jaemyung ^{[5
]}

Chen, Yu-Jen ^{[1
]}

Smith, Brian ^{[2
]}

Pepper, John S. ^{[2
]}

Shao, Yu-Cheng ^{[1
,6
]}

Huang, Shih-Wen ^{[7
]}

Wray, L. Andrew ^{[8
]}

Gullikson, E. ^{[9
]}

Shen, Zhi-Xun ^{[4
,10
]}

Devereaux, Thomas P. ^{[4
]}

Tremsin, Anton ^{[11
]}

Yang, Wanli ^{[1
]}

Guo, Jinghua ^{[1
]}

Duarte, Robert ^{[2
]}

Hussain, Zahid ^{[1
]}

机构：

[1] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA

[2] Lawrence Berkeley Natl Lab, Engn Div, Berkeley, CA 94720 USA

[3] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA

[4] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[5] Natl Inst Mat Sci NIMS, Res Ctr Adv Measurement & Characterizat, Synchrotron X ray Grp, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan

[6] Tamkang Univ, Dept Phys, New Taipei City 25137, Taiwan

[7] Lund Univ, MAX Lab 4, POB 118, S-22100 Lund, Sweden

[8] NYU, Dept Phys, New York, NY 10003 USA

[9] Lawrence Berkeley Natl Lab, Ctr X ray Opt, Berkeley, CA 94720 USA

[10] Stanford Univ, Dept Phys, Stanford, CA 94305 USA

[11] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA

来源：

JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA | 2022年 / 257卷

关键词：

Resonant inelastic X-ray scattering; Modular X-ray spectrometer; SPECTROMETER; BEAMLINE; DESIGN;

D O I：

10.1016/j.elspec.2019.146897

中图分类号：

O433 [光谱学];

学科分类号：

0703 ; 070302 ;

摘要：

A momentum resolved resonant inelastic X-ray scattering (qRIXS) experimental station with continuously rotatable spectrometers and parallel detection is designed to operate at different beamlines at synchrotron and free electron laser (FEL) facilities. This endstation, currently located at the Advanced Light Source (ALS), has five emission ports on the experimental chamber for mounting the high-throughput modular soft X-ray spectrometers (MXS) [24]. Coupled to the rotation from the supporting hexapod, the scattered X-rays from 27.5 degrees (forward scattering) to 152.5 degrees (backward scattering) relative to the incident photon beam can be recorded, enabling the momentum-resolved RIXS spectroscopy. The components of this endstation are described in details, and the preliminary RIXS measurements on highly oriented pyrolytic graphite (HOPG) reveal the low energy vibronic excitations from the strong electron-phonon coupling at C K edge around sigma* band. The grating upgrade option to enhance the performance at low photon energies is presented and the potential of this spectroscopy is discussed in summary.

引用

页数：7

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