On Resonant Scatterers As a Factor Limiting Carrier Mobility in Graphene

被引:209
作者
Ni, Z. H. [1 ]
Ponomarenko, L. A. [1 ]
Nair, R. R. [1 ]
Yang, R. [1 ]
Anissimova, S. [1 ]
Grigorieva, I. V. [1 ]
Schedin, F. [1 ]
Blake, P. [1 ]
Shen, Z. X. [2 ]
Hill, E. H. [1 ]
Novoselov, K. S. [1 ]
Geim, A. K. [1 ]
机构
[1] Univ Manchester, Ctr Mesosci & Nanotechnol, Manchester M13 9PL, Lancs, England
[2] Nanyang Technol Univ, Sch Phys & Math Sci, Singapore 637371, Singapore
基金
英国工程与自然科学研究理事会;
关键词
Graphene; mobility; scattering mechanism; Raman; RAMAN-SPECTROSCOPY; TRANSPORT;
D O I
10.1021/nl101399r
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We show chat graphene deposited on a substrate has a non-negligible density of atomic scale defects This is evidenced by a previously unnoticed D peak in the Raman spectra with intensity of similar to 1 % with respect to the G peak We evaluated the effect of such impurities on electron transport by mimicking them with hydrogen adsorbates and measuring the induced changes in both mobility and Raman intensity If the intervalley scatterers responsible for the D peak are monovalent, their concentration is sufficient to account for the limited mobilities currently achievable in graphene on a substrate
引用
收藏
页码:3868 / 3872
页数:5
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