Self diffusion in liquid aluminium

被引:81
作者
Kargl, F. [1 ]
Weis, H. [1 ]
Unruh, T.
Meyer, A. [1 ]
机构
[1] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Mat Phys Weltraum, D-51170 Cologne, Germany
来源
5TH EUROPEAN CONFERENCE ON NEUTRON SCATTERING | 2012年 / 340卷
关键词
SCATTERING; DENSITY; METALS;
D O I
10.1088/1742-6596/340/1/012077
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Here we report temperature dependent self-diffusion coefficients of liquid aluminium measured on absolute scale by using incoherent quasielastic neutron scattering at temperatures of 980K, 1020K, and 1060K. Aluminium self-diffusion coefficients follow an Arrhenius law with an activation energy of 280 +/- 70 meV. The Sutherland-Einstein equation relating viscosity to the diffusion coefficient well captures the temperature dependence and absolute values of the here reported aluminium self-diffusion coefficients using the covalent radius of aluminium. A comparison to published molecular dynamics simulation data helps to further narrow down the choice of the potential.
引用
收藏
页数:5
相关论文
共 19 条
  • [1] Reference data for the density and viscosity of liquid aluminum and liquid iron
    Assael, MJ
    Kakosimos, K
    Banish, RM
    Brillo, J
    Egry, I
    Brooks, R
    Quested, PN
    Mills, KC
    Nagashima, A
    Sato, Y
    Wakeham, WA
    [J]. JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 2006, 35 (01) : 285 - 300
  • [2] Atomistic comparison of volume-dependent melt properties from four models of aluminum
    Becker, C. A.
    Kramer, M. J.
    [J]. MODELLING AND SIMULATION IN MATERIALS SCIENCE AND ENGINEERING, 2010, 18 (07)
  • [3] SOUND-VELOCITY AND COMPRESSIBILITY IN LIQUID-METALS
    BLAIRS, S
    JOASOO, U
    [J]. JOURNAL OF INORGANIC & NUCLEAR CHEMISTRY, 1980, 42 (11): : 1555 - 1558
  • [4] CALCULATION OF DYNAMICAL STRUCTURE FACTOR FOR LIQUID ALUMINUM
    EBBSJO, I
    KINELL, T
    WALLER, I
    [J]. JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 1978, 11 (13): : L501 - L504
  • [5] Improvement of computer simulation models for metallic melts via quasielastic neutron scattering: A case study of liquid titanium
    Horbach, J.
    Rozas, R. E.
    Unruh, T.
    Meyer, A.
    [J]. PHYSICAL REVIEW B, 2009, 80 (21)
  • [6] Iida T., 1993, PHYS PROPERTIES LIQU
  • [7] In situ studies of mass transport in liquid alloys by means of neutron radiography
    Kargl, F.
    Engelhardt, M.
    Yang, F.
    Weis, H.
    Schmakat, P.
    Schillinger, B.
    Griesche, A.
    Meyer, A.
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2011, 23 (25)
  • [8] KASPEROVICH G, 2010, INT FOUNDRY RES, V4, P2
  • [9] Mehrer H., 2007, DIFFUSION SOLIDS
  • [10] Meyer A, 2002, PHYS REV B, V66, DOI 10.1103/PhysRevB.66.134205