Carbon Dioxide Reforming of Methane to Syngas by Thermal Plasma

被引:7
作者
Sun Yanpeng [1 ]
Nie Yong [1 ]
Wu Angshan [1 ]
Ji Dengxiang [1 ]
Yu Fengwen [1 ]
Ji Jianbing [1 ]
机构
[1] Zhejiang Univ Technol, Coll Chem Engn & Mat Sci, Hangzhou 310014, Peoples R China
关键词
thermal plasma; methane; carbon dioxide; syngas; reforming; CONVERSION;
D O I
10.1088/1009-0630/14/3/12
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
Experiments were conducted on syngas preparation from dry reforming of methane by carbon dioxide with a DC arc plasma at atmospheric pressure. In all experiments, nitrogen gas was used as the working. gas for thermal plasma to generate a high-temperature jet into a horizontal tube reactor. A mixture of methane and carbon dioxide was fed vertically lino the jet. In order to obtain a higher conversion rate of methane and carbon dioxide, chemical energy efficiency and fuel production efficiency, parametric screening studies were conducted, in which the volume ratio of carbon dioxide to methane in fed gases and the total flux of fed gases were taken into account, Results showed that carbon dioxide reforming of methane to syngas by thermal plasma exhibited a larger processing capacity, higher conversion of methane and carbon dioxide and higher chemical energy efficiency and fuel production efficiency. In addition, thermodynamic simulation for the reforming process was conducted Experimental data agreed well with the thermodynamic results. indicating that high thermal efficiency can he achieved with the thermal plasma reforming process.
引用
收藏
页码:252 / 256
页数:5
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