Beryllium-7 Elucidate Sediment Dynamics of the Branford River Estuary, Connecticut, USA

被引:3
作者
Benoit, Gaboury [1 ]
Hirschbeck, Matthew [2 ]
Bisson, Beth [3 ]
机构
[1] Yale Environm Sch, 195 Prospect St, New Haven, CT 06511 USA
[2] Natl Pk Serv Intermt Reg, 12795 W Alameda Pkwy, Lakewood, CO 80228 USA
[3] Univ Maine, Maine Sea Grant Coll Program, 5741 Libby Hall, Orono, ME 04469 USA
关键词
Estuary; Beryllium-7; Mass balance; Pollution; Scavenging; Rivers; Watershed; Sediments; Deposition; Resuspension; UNITED-STATES; BE-7; RADIONUCLIDES; TRANSPORT; PB-210; GEOCHEMISTRY; VARIABILITY; DEPOSITION; PARTICLES; TRACERS;
D O I
10.1007/s12237-020-00712-5
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Berrylium-7 elucidates sediment dynamics (i.e., sources, sinks, deposition, and resuspension) in a Connecticut estuary. Average annual atmospheric deposition of Be-7 is 290 mBq cm(-2) year(-1). Sediment samples from 43 locations within the estuary show that Be-7 deposition is spatially complex, but were statistically indistinguishable a year apart. Weekly time series of sediments indicate that levels are nearly constant on this shorter time scale once radioactive decay is taken into account. Be-7 levels in sediments are a balance between steady losses through radioactive decay and periodic pulse inputs following rainstorms. The water column was measured intensively during three rain events, showing that Be-7 is removed rapidly from the water column, with a rate constant averaging 1.00 +/- 0.12 day(-1). A mass balance shows that Be-7 is supplied about equally by direct precipitation onto the estuary's surface and inflow from the watershed. Losses from the water column are split between net sedimentation (43%) and tidal flushing (57%). Variations in sedimentary Be-7 levels at very short (meters) and longer (km) distances, and changes at time scales from hours to years, indicate that a large number of samples are required to capture all the variability in these highly dynamic systems. The current study differs from previous research in that a large number of measurements were conducted on a smaller system, and a full mass balance was developed.
引用
收藏
页码:831 / 842
页数:12
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