Characterization of fine and carbonaceous particles emissions from pelletized biomass-coal blends combustion: Implications on residential crop residue utilization in China

被引:28
作者
Xu, Yue [2 ]
Wang, Yan [3 ]
Chen, Yingjun [1 ]
Tian, Chongguo [4 ]
Feng, Yanli [5 ]
Li, Jun [6 ]
Zhang, Gan [6 ]
机构
[1] Tongji Univ, China Meteorol Adm, Coll Environm Sci & Engn,Key Lab Cities Mitigat &, State Key Lab Pollut Control & Resources Reuse, Shanghai 200092, Peoples R China
[2] Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550081, Peoples R China
[3] Dalian Univ Technol, Sch Environm Sci & Technol, Key Lab Ind Ecol & Environm Engn MOE, Dalian 116024, Peoples R China
[4] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
[5] Shanghai Univ, Inst Environm Pollut & Hlth, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
[6] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
关键词
PM2.5; OC; EC; Biomass pellets; Pelletized biomass-coal blends; POLYCYCLIC AROMATIC-HYDROCARBONS; HOUSEHOLD BIOFUEL COMBUSTION; PARTICULATE MATTER; FIELD MEASUREMENT; RURAL CHINA; FUEL; STOVES; EC; OC; PM;
D O I
10.1016/j.atmosenv.2016.06.073
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Bulk biofuel, biomass pellets and pelletized biomass-coal blends were combusted in a typical rural conventional household stove and a high-efficiency stove. Reductions in PM2.5, organic carbon (OC) and elemental carbon (EC) emissions were evaluated by comparing emission factors (EFs) among 19 combinations of biofuel/residential stove types measured using a dilution sampling system. In the low efficiency stove, the average EFs of PM2.5, OC, and EC of biomass pellets were 2.64 +/- 1.56, 0.42 +/- 0.36, and 0.30 +/- 0.11 g/kg, respectively, significantly lower than those burned in bulk form. EFPM2.5 and EFOC of pelletized biomass combustion in the high-efficiency stove were lower than those of the same biofuel burned in the low-efficiency stove. Furthermore, pelletized corn residue and coal blends burned in the high-efficiency stove could significantly decrease emissions. Compared with the bulk material burned in the low-efficiency stove, the reduction rates of PM2.5, OC and EC from pelletized blends in the high-efficiency stove can reach 84%, 96% and 93%, respectively. If the annually produced corn residues in 2010 had been blended with 10% anthracite coal powder and burnt as pellets, it would have reduced about 82% of PM2.5, 90-96% of OC and 81-92% of EC emission in comparison with burning raw materials in conventional household stoves. Given the low cost, high health benefit and reduction effect on atmospheric pollutants, pelletized blends could be a promising alternative to fossil fuel resources or traditional bulk biofuel. (C) 2016 Elsevier Ltd. All rights reserved.
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页码:312 / 319
页数:8
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