Specific Recognition of Uranyl Ion Employing a Functionalized Nanochannel Platform for Dealing with Radioactive Contamination

被引:29
作者
Yang, Linsen [2 ,3 ]
Ban, Yongchao [4 ]
Kong, Xiang-Yu [2 ]
Si, Mengting [1 ]
Zhao, Yuanyuan [2 ]
Niu, Bo [2 ,3 ]
Zhao, Xiaolu [2 ]
Wei, Yan [1 ]
Jiang, Lei [2 ,3 ]
Wen, Liping [2 ,3 ]
机构
[1] Peking Univ Sch & Hosp Stomatol, Dept Geriatr Dent, Beijing Lab Biomed Mat, Beijing 100081, Peoples R China
[2] Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Bioinspired Mat & Interfacial Sci, Beijing 100190, Peoples R China
[3] Univ Chinese Acad Sci, Sch Future Technol, Beijing 100049, Peoples R China
[4] Northwestern Polytech Univ, Sch Sci, Shanxi Key Lab Macromol Sci & Technol, Xian 710072, Peoples R China
基金
中国国家自然科学基金; 北京市自然科学基金; 国家重点研发计划;
关键词
specific recognition; uranyl cation; functionalized nanochannel; ultralow-concentration detection; remove radioactive contamination; COLORIMETRIC DETECTION; URANIUM ADSORPTION; CARBON DOTS; UO22+; AMPLIFICATION; THORIUM; SENSOR; SPECTROSCOPY; LANTHANIDES; FABRICATION;
D O I
10.1021/acsami.9b19544
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Radioactive contamination is a highly concerning global environmental issue along with the development of the nuclear industry. On account of sophisticated operations and high cost of instrument detection methods, numerous efforts have been focused on rapid and simple detection of pollution elements and uranium is the most common one. It is an enormous challenge to push the limit of determination as low as possible while carrying out ultrasensitive detection. Here, we report an intelligent platform based on functionalized solid nanochannels to monitor ultratrace uranyl ions. The platform has a detection limit of 1 fM, which is far below the value that traditional instrumental methods can reach. What is more, the system also exhibits uranyl removal property. The mesenchymal stem cells cultivated in media containing uranyl can achieve excellent viability in the presence of the membranes. This work provides a new choice for handling global radioactive contamination of water.
引用
收藏
页码:3854 / 3861
页数:8
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