Flaring emissions in Africa: Distribution, evolution and comparison with current inventories

被引:21
作者
Doumbia, El Hadji Thierno [1 ]
Liousse, Catherine [2 ]
Keita, Sekou [3 ]
Granier, Louise [4 ]
Granier, Claire [2 ,5 ,6 ]
Elvidge, Christopher D. [7 ]
Elguindi, Nellie [2 ]
Law, Kathy [4 ]
机构
[1] Meteo France, Ctr Natl Rech Meteorol, Toulouse, France
[2] Univ Toulouse, CNRS, Lab Aerol, Toulouse, France
[3] Univ Felix Houphouet Boigny, Lab Phys Atmosphere, Abidjan, Cote Ivoire
[4] Univ Sorbonne, CNRS, Lab Atmospheres Milieux Observat Spatiales, Paris, France
[5] NOAA, Earth Syst Res Lab, Div Chem Sci, Boulder, CO USA
[6] Cooperat Inst Res Environm Sci, Boulder, CO USA
[7] NOAA, Earth Observat Grp, Natl Ctr Environm Informat, Boulder, CO USA
关键词
Defense meteorological satellite program (DMSP); Nighttime light; Emission factor; Flare; Chemical compounds; Africa; BLACK CARBON; ANTHROPOGENIC EMISSIONS; GAS; POLLUTION;
D O I
10.1016/j.atmosenv.2018.11.006
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Flaring emissions are a major concern due to large uncertainties in the amount of chemical compounds released into the atmosphere and their evolution with time. A methodology based on DMSP (Defense Meteorological Satellite Program) nighttime light data combined with regional gas flaring volumes from National Oceanic and Atmospheric Administration's National Centers for Environmental Information (NOAA-NCEI) has been developed to estimate flaring emissions. This method is validated in Nigeria where individual field company data are available. The spatial distribution of CO2, CH4, NMVOCs, CO, OC, BC, SO2 and NOx is derived for the African continent for the period 1995-2010. A range of the emissions due to flaring is estimated based on the range of emission factors (EFs) for each chemical species. An average decrease in CO2 emissions of about 30% is found over Africa from 1995 to 2010, with Nigeria being the largest contributor to this reduction (up to 50%). Changes in the spatial distribution with time indicate local increases, particularly at offshore platforms, which are attributed to a lack of regulations as well as aging infrastructures in oil and gas fields. Comparisons with current inventories reveal differences in the location and magnitude of point source emissions. For chemical compounds such as NMVOCs and CH4, the ECLIPSE and EDGAR country-level values are considerably higher than the highest flaring emission estimated in this study for 2005. For species such as CO, OC, BC, SO2 and NOx the emissions provided by the ECLIPSE and EDGAR inventories are generally within the same order of magnitude as the average values found in this study, with the exception of OC, BC and SO2 in which EDGAR provides much lower emissions. These discrepancies are likely due to either differences in the methodologies used to estimate the emissions, in the values of the emission factors considered, or in the definition of flaring sector. Our current estimations suggest that BC, CH4 and CO2 flaring emissions in Africa account for 1-15% (on average 7%), 0.5-8% (on average 2%) and 8-13% (on average 11%) of African total anthropogenic emissions, respectively. The contribution of flaring to African anthropogenic emissions varies widely among countries. For example, in Nigeria the average emissions due to flaring are estimated to be as high as 18% for BC, 10% for CH4 and 50% for CO2, which is significantly greater than the continental average and highlights the importance of emissions in flaring areas.
引用
收藏
页码:423 / 434
页数:12
相关论文
共 39 条
[1]  
Allen D.T., 2011, TCEQ 2010 Flare Study Final Report - Appendices
[2]  
Canadian Association of Petroleum Producers, 2014, NPRI GUID REC APPR C
[3]  
CONCAWE, 2009, 109 CONCAWE
[4]   The major sources of gas flaring and air contamination in the natural gas processing plants: A case study [J].
Davoudi, M. ;
Rahimpour, M. R. ;
Jokar, S. M. ;
Nikbakht, F. ;
Abbasfard, H. .
JOURNAL OF NATURAL GAS SCIENCE AND ENGINEERING, 2013, 13 :7-19
[5]  
Deetz K, 2016, GEOSCI MODEL DEV DIS, P1, DOI [10.5194/gmd-2016-110, DOI 10.5194/GMD-2016-110]
[6]  
E&P Forum, 1994, 259197 E P FOR OIL I
[7]  
Elvidge CD, 2007, OIL GAS J, V105, P50
[8]   A Fifteen Year Record of Global Natural Gas Flaring Derived from Satellite Data [J].
Elvidge, Christopher D. ;
Ziskin, Daniel ;
Baugh, Kimberly E. ;
Tuttle, Benjamin T. ;
Ghosh, Tilottama ;
Pack, Dee W. ;
Erwin, Edward H. ;
Zhizhin, Mikhail .
ENERGIES, 2009, 2 (03) :595-622
[9]  
ESRI, 2016, ArcGis Desktop: Release 10.4
[10]   Detection of a gas flaring signature in the AERONET optical properties of aerosols at a tropical station in West Africa [J].
Fawole, Olusegun G. ;
Cai, Xiaoming ;
Levine, James G. ;
Pinker, Rachel T. ;
MacKenzie, A. R. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2016, 121 (24) :14513-14524